degradation;
electrochemical advanced oxidisation process (EAOP);
emerging contaminants;
per- and polyfluoroalkyl substances (PFASs);
persistent organic pollutants;
BORON-DOPED DIAMOND;
PERFLUOROOCTANE SULFONATE PFOS;
GLOBAL EMISSION INVENTORIES;
WASTE-WATER TREATMENT;
IN-SITU REMEDIATION;
ACID PFCA HOMOLOGS;
EMERGING CONTAMINANTS;
AQUEOUS-SOLUTION;
FILM ELECTRODES;
POLYFLUOROALKYL SUBSTANCES;
D O I:
10.1515/jaots-2017-0014
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Per- and polyfluoroalkyl substances (PFASs) have been recently listed as emerging contaminants (ECs) and persistent organic pollutants (POPs) due to their human and environmental health concerns. In the last 10 years, their detection and remediation have progressed significantly. Herein, we critically review recent developments in electrochemical advanced oxidation process (EAOP) towards their remediation. Particular attentions are paid to perfluorooctane sulfonate (PFOS) and perfluorooctanoic acid (PFOA), which present the main concerns of PFASs at this time. Due to the persistence of those PFASs, other remediation approaches may experience difficulty in degrading them, whilst EAOP has demonstrated success. The fundamentals of EAOP are highlighted and the scale-up application is discussed regarding the future research directions.