The simultaneous capture of mercury and fine particles by hybrid filter with powder activated carbon injection

被引:18
作者
Jang, Ha-Na [1 ]
Back, Seung-Ki [1 ]
Sung, Jin-Ho [1 ]
Kang, Youn-Suk [2 ]
Jurng, Jongsoo [3 ]
Seo, Yong-Chil [1 ]
机构
[1] Yonsei Univ, Dept Environm Engn, Wonju 220710, South Korea
[2] JE Tech Co Ltd, R&D Ctr, Seoul 153813, South Korea
[3] Korea Inst Sci & Technol, Ctr Environm Hlth & Welf Res, Seoul 02792, South Korea
关键词
Powder activated carbon; Hybrid filter; Fine particulate matter; Elemental mercury; Particulate mercury; FLUE-GAS; FLY-ASH; COAL; EMISSIONS; REMOVAL; COMBUSTION; OXIDATION;
D O I
10.1016/j.envpol.2018.02.080
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The hybrid filter (HF) was newly designed and operated with powder activated carbon (PAC) injection to capture mercury and fine particulate matter in the coal power plant. With PAC injection in HF operation, the capture efficiency of elemental mercury was clearly enhanced. When the injection rate of PAC increased from 0 to 20 mg/m(3), the speciation fraction of elemental mercury significantly decreased from 85.19% to 3.76% at the inlet of the hybrid filter. The speciation fraction of oxidized mercury did not vary greatly, whereas the particulate mercury increased from 1.31% to 94.04%. It was clearly observed that the HF played a role in the capture of mercury and fine PM by leading the conversion of elemental mercury as particulate mercury and the growth of PM via electrode discharge in the HF operation with PAC injection. (C) 2018 Elsevier Ltd. All rights reserved.
引用
收藏
页码:531 / 540
页数:10
相关论文
共 31 条
[1]  
Air Pollution Prevention and Control Division National Risk Management Research Laboratory US Environmental Protection Agency, 2005, CONTR MERC EM COAL F
[2]   Control of mercury emissions from coal-fired power plants: a preliminary cost assessment and the next steps for accurately assessing control costs [J].
Brown, TD ;
Smith, DN ;
O'Dowd, WJ ;
Hargis, RA .
FUEL PROCESSING TECHNOLOGY, 2000, 65 :311-341
[3]   Fixed-bed studies of the interactions between mercury and coal combustion fly ash [J].
Dunham, GE ;
DeWall, RA ;
Senior, CL .
FUEL PROCESSING TECHNOLOGY, 2003, 82 (2-3) :197-213
[4]  
Energy & Environmental Research Center, 2004, ATM MERC RES UPD
[5]  
Energy & Environmental Research Center, COMPR EV FLUE GAS ME
[6]   Mercury transformations in coal combustion flue gas [J].
Galbreath, KC ;
Zygarlicke, CJ .
FUEL PROCESSING TECHNOLOGY, 2000, 65 :289-310
[7]   Mercury capture by native fly ash carbons in coal-fired power plants [J].
Hower, James C. ;
Senior, Constance L. ;
Suuberg, Eric M. ;
Hurt, Robert H. ;
Wilcox, Jennifer L. ;
Olson, Edwin S. .
PROGRESS IN ENERGY AND COMBUSTION SCIENCE, 2010, 36 (04) :510-529
[8]   Mercury Oxidation over the V2O5(WO3)/TiO2 Commercial SCR Catalyst [J].
Kamata, Hiroyuki ;
Ueno, Shun-ichiro ;
Naito, Toshiyuki ;
Yukimura, Akinori .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2008, 47 (21) :8136-8141
[9]  
Keating M. H., 1997, EXECUTIVE SUMMARY ME, V1
[10]  
Kilgroe J.D. S., 2001, Control of mercury emissions from coal-fired electric utility boilers: interim report