Facile one-pot green synthesis of magnetic separation photocatalyst-adsorbent and its application

被引:77
作者
Cheng, Song [1 ,2 ]
Zhao, Saidan [1 ]
Xing, Baolin [1 ,2 ]
Shi, Changliang [1 ]
Meng, Weibo [1 ]
Zhang, Chuanxiang [1 ,2 ]
Bo, Zhang [3 ]
机构
[1] Henan Polytech Univ, Coll Chem & Chem Engn, Jiaozuo 454003, Peoples R China
[2] Collaborat Innovat Ctr Coal Work Safety & Clean Hi, Jiaozuo 454003, Peoples R China
[3] China Univ Min & Technol, Key Lab Coal Proc & Efficient Utilizat, Minist Educ, Xuzhou 221116, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
Adsorption; Dye wastewater; Magnetic separation photocatalyst-adsorbent; One-pot; Photocatalytic activity; WASTE-WATER; ACTIVATED CARBON; MALACHITE GREEN; CATIONIC DYES; ZNO; ADSORPTION; REMOVAL; DEGRADATION; NANOCOMPOSITES; KINETICS;
D O I
10.1016/j.jwpe.2022.102802
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Magnetic separation photocatalyst-adsorbent (MSPA) is successfully prepared by pyrolysis of cotton stem for rhodamine B and malachite green wastewater removal using one-pot method. The results show that MSPA has the property of magnetism, photocatalytic degradation and adsorption. The adsorption isotherms and adsorption kinetics of rhodamine B and malachite green are determined. The maximum adsorption amounts of the Rhodamine B and malachite green are 475.49 mg/g and 646.82 mg/g, respectively. The photodegradation removals of rhodamine B and malachite green are close to 1, which is attributed to the adsorption performance of MSPA, and synergy between adsorption and photodegradation. The photocatalytic degradation mechanism is detailed investigated. MSPA can be quickly recycled from aqueous solution under extra magnetic field after use. The present work demonstrates that the waste cotton stem is converted into promising MSPA for dye wastewater removal.
引用
收藏
页数:10
相关论文
共 51 条
[1]   Zero-valent iron supported-lemon derived biochar for ultra-fast adsorption of methylene blue [J].
Abd El-Monaem, Eman M. ;
Omer, Ahmed M. ;
El-Subruiti, Gehan M. ;
Mohy-Eldin, Mohamed S. ;
Eltaweil, Abdelazeem S. .
BIOMASS CONVERSION AND BIOREFINERY, 2024, 14 (02) :1697-1709
[2]   Kinetics and thermodynamics of Malachite Green dye removal from aqueous phase using iron nanoparticles loaded on ash [J].
Agarwal, Shilpi ;
Tyagi, Inderjeet ;
Gupta, Vinod Kumar ;
Mashhadi, Somaye ;
Ghasemi, Maryam .
JOURNAL OF MOLECULAR LIQUIDS, 2016, 223 :1340-1347
[3]   Defect induced ferromagnetism in carbon-doped ZnO thin films [J].
Akbar, Sadaf ;
Hasanain, S. K. ;
Abbas, Manzar ;
Ozcan, S. ;
Ali, B. ;
Shah, S. Ismat .
SOLID STATE COMMUNICATIONS, 2011, 151 (01) :17-20
[4]   Potential use of alkaline treated algae waste biomass as sustainable biosorbent for clean recovery of cadmium(II) from aqueous media: batch and column studies [J].
Bulgariu, Dumitru ;
Bulgariu, Laura .
JOURNAL OF CLEANER PRODUCTION, 2016, 112 :4525-4533
[5]   Enhancement of Rhodamine B removal by low-cost fly ash sorption with Fenton pre-oxidation [J].
Chang, Shih-Hsien ;
Wang, Kai-Sung ;
Li, Heng-Ching ;
Wey, Ming-Yen ;
Chou, Jing-Dong .
JOURNAL OF HAZARDOUS MATERIALS, 2009, 172 (2-3) :1131-1136
[6]   Preparation and Characterization of ZnO Nanoparticles Supported on Amorphous SiO2 [J].
Chen, Ying ;
Ding, Hao ;
Sun, Sijia .
NANOMATERIALS, 2017, 7 (08)
[7]   High-efficiency removal of lead/cadmium from wastewater by MgO modified biochar derived from crofton weed [J].
Cheng, Song ;
Zhao, Saidan ;
Guo, Hui ;
Xing, Baolin ;
Liu, Yongzhi ;
Zhang, Chuanxiang ;
Ma, Mingjie .
BIORESOURCE TECHNOLOGY, 2022, 343
[8]   Lead and cadmium clean removal from wastewater by sustainable biochar derived from poplar saw dust [J].
Cheng, Song ;
Liu, Yongzhi ;
Xing, Baolin ;
Qin, Xiaojing ;
Zhang, Chuangxiang ;
Xia, Hongying .
JOURNAL OF CLEANER PRODUCTION, 2021, 314
[9]   Efficient and selective removal of Pb(II) from aqueous solution by modification crofton weed: Experiment and density functional theory calculation [J].
Cheng, Song ;
Xing, Baolin ;
Shi, Changliang ;
Nie, Yanhe ;
Xia, Hongying .
JOURNAL OF CLEANER PRODUCTION, 2021, 280
[10]   Microwave-assisted catalytic pyrolysis of the Eupatorium adenophorum for obtaining valuable products [J].
Cheng, Song ;
Zhang, Qi ;
Shu, Jianhua ;
Xia, Hongying ;
Zhang, Libo ;
Peng, Jinhui ;
Lin, Guo ;
Hu, Wenhai ;
Chen, Quan .
ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY, 2020, 39 (05)