Nickel(0)-Catalyzed Enantioselective Annulations of Alkynes and Arylenoates Enabled by a Chiral NHC Ligand: Efficient Access to Cyclopentenones

被引:49
作者
Ahlin, Joachim S. E. [1 ]
Donets, Pavel A. [1 ]
Cramer, Nicolai [1 ]
机构
[1] EPFL SB ISIC LCSA, Lab Asymmetr Catalysis & Synth, CH-1015 Lausanne, Switzerland
基金
瑞士国家科学基金会;
关键词
annulation; asymmetric catalysis; carbenes; cyclopentenones; nickel; PAUSON-KHAND REACTION; HETEROCYCLIC CARBENE LIGANDS; COMPLEXES SYNTHESIS; COUPLING REACTIONS; NAZAROV CYCLIZATIONS; REDUCTIVE COUPLINGS; ALLYLIC ALCOHOLS; PROSTAGLANDINS; CYCLOADDITION; DERIVATIVES;
D O I
10.1002/anie.201408364
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Cyclopentenones are versatile structural motifs of natural products as well as reactive synthetic intermediates. The nickel-catalyzed reductive [3+2] cycloaddition of alpha,beta-unsaturated aromatic esters and alkynes constitutes an efficient method for their synthesis. Here, nickel(0) catalysts comprising a chiral bulky C-1-symmetric N-heterocyclic carbene ligand were shown to enable an efficient asymmetric synthesis of cyclopentenones from mesityl enoates and internal alkynes under mild conditions. The bulky NHC ligand provided the cyclopentenone products in very high enantioselectivity and led to a regioselective incorporation of unsymmetrically substituted alkynes.
引用
收藏
页码:13229 / 13233
页数:5
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