Piezocatalytic performance difference of graphitic carbon nitride (g-C3N4) derived from different precursors

被引:31
作者
Shao, Yuqiu [1 ]
Liu, Chengcan [1 ]
Ma, Huirong [1 ]
Chen, Jingjing [1 ]
Dong, Chenlong [1 ]
Wang, Dajian [1 ]
Mao, Zhiyong [1 ]
机构
[1] Tianjin Univ Technol, Sch Mat Sci & Engn, Sch Sci, Tianjin 300384, Peoples R China
关键词
Piezocatalysis; Graphitic carbon nitride; Pollutant degradation; Reactive oxygen species; DOPED G-C3N4; BAND-GAP; LIGHT; PIEZO; WATER; PHOTOCATALYSTS; ENHANCEMENT; EVOLUTION; VACANCY; ENERGY;
D O I
10.1016/j.cplett.2022.139748
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this paper, four types of graphitic carbon nitride (g-C3N4) are prepared from different precursors by thermal polycondensation method and the piezocatalytic performance difference of the obtained g-C(3)N(4 )materials are investigated in detail. g-C(3)N(4 )derived from thiourea delivers best piezocatalytic performance basing on KMnO4 reduction experiment and rhodamine B degradation experiment. According to the differences of piezocatalytic performance of these g-C(3)N(4 )materials, effects of morphology, composition and defects on piezocatalytic performances are discussed. Reactive oxygen species (ROS) capture experiment showed that g-C(3)N(4 )could produce ROS through piezoelectric effect and hydroxyl radical (& BULL;OH) played a major role in pollutant degradation.
引用
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页数:12
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