Novel excitations near quantum criticality in geometrically frustrated antiferromagnet CsFeCl3

被引:15
作者
Hayashida, Shohei [1 ,6 ]
Matsumoto, Masashige [2 ]
Hagihala, Masato [1 ,7 ]
Kurita, Nobuyuki [3 ]
Tanaka, Hidekazu [3 ]
Itoh, Shinichi [4 ]
Hong, Tao [5 ]
Soda, Minoru [1 ,8 ]
Uwatoko, Yoshiya [1 ]
Masuda, Takatsugu [1 ]
机构
[1] Univ Tokyo, Inst Solid State Phys, Chiba 2778581, Japan
[2] Shizuoka Univ, Dept Phys, Shizuoka 4228529, Japan
[3] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan
[4] High Energy Accelerator Res Org, Inst Mat Struct Sci, Neutron Sci Div, Tsukuba, Ibaraki 3050801, Japan
[5] Oak Ridge Natl Lab, Neutron Scattering Div, Oak Ridge, TN 37831 USA
[6] Swiss Fed Inst Technol, Solid State Phys Lab, Zurich, Switzerland
[7] High Energy Accelerator Res Org, Inst Mat Struct Sci, Tsukuba, Ibaraki, Japan
[8] RIKEN, Ctr Emergent Matter Sci, Wako, Saitama, Japan
基金
日本学术振兴会;
关键词
NEUTRON-SCATTERING SPECTRA; HIGGS AMPLITUDE MODE; PHASE; MAGNETISM; STATE;
D O I
10.1126/sciadv.aaw5639
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The investigation of materials that exhibit quantum phase transition provides valuable insights into fundamental problems in physics. We present neutron scattering under pressure in a triangular-lattice antiferromagnet that has a quantum disorder in the low-pressure phase and a noncollinear structure in the high-pressure phase. The neutron spectrum continuously evolves through critical pressure; a single mode in the disordered state becomes soft with the pressure and it splits into gapless and gapped modes in the ordered phase. Extended spin-wave theory reveals that the longitudinal and transverse fluctuations of spins are hybridized in the modes because of noncollinearity, and previously unidentified magnetic excitations are formed. We report a new hybridization of the phase and amplitude fluctuations of the order parameter near a quantum critical point in a spontaneously symmetry-broken state.
引用
收藏
页数:5
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