Enhanced Light Harvesting and Electron Lifetime of Front Side-illuminated CdSe Quantum Dot-assembled TiO2 Nanotube Arrays for Quantum Dot-sensitized Solar Cells

被引:2
作者
Jung, Sung Woo [1 ]
Lee, Soo-Yong [1 ]
Park, Min-Ah [1 ]
Kim, Jae-Hong [1 ]
Kang, Soon-Hyung [2 ]
Kim, Hyunsoo [3 ]
Choi, Chel-Jong [3 ]
Ahn, Kwang-Soon [1 ]
机构
[1] Yeungnam Univ, Sch Chem Engn, Gyongsan 712749, South Korea
[2] Chonnam Natl Univ, Dept Chem Educ, Kwangju, South Korea
[3] Chonbuk Natl Univ, Sch Semicond & Chem Engn, Jeonju 561756, South Korea
基金
新加坡国家研究基金会;
关键词
light harvesting; front side illumination; quantum dot-sensitized solar cell; electron lifetime; nanotube array; DYE; EFFICIENCY; FILMS;
D O I
10.1080/15421406.2014.933386
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
CdSe quantum dots (QDs)-assembled, free-standing TiO2 nanotube arrays (TNTs) are transferred to transparent fluorine-doped tin oxides (FTOs) using a sol-gel process. The TNTs on the FTO (FTO/TNT) not only provide an efficient 1-dimensional electron pathway with few recombination centers, but also allow front side illumination through the transparent FTO, providing a significantly enhanced electron lifetime and light harvesting compared to conventional TNTs on Ti foil and TiO2 nanoparticles-based mesoporous films on the FTO. These effects help improve significantly the short circuit current and open-circuit voltage of quantum dot-sensitized solar cells (QD-SSCs).
引用
收藏
页码:144 / 153
页数:10
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