Facile fabrication of Bi2S3/SnS2 heterojunction photocatalysts with efficient photocatalytic activity under visible light

被引:90
作者
Gao, Xiaomin [1 ]
Huang, Guanbo [1 ]
Gao, Haihuan [2 ]
Pan, Cheng [1 ]
Wang, Huan [1 ]
Yan, Jing [1 ,3 ]
Liu, Yu [1 ]
Qiu, Haixia [1 ,3 ]
Ma, Ning [1 ]
Gao, Jianping [1 ,3 ]
机构
[1] Tianjin Univ, Sch Sci, Dept Chem, Tianjin 300072, Peoples R China
[2] Tianjin Fourth Middle Sch, Tianjin 300021, Peoples R China
[3] Collaborat Innovat Ctr Chem Sci & Engn, Tianjin 300072, Peoples R China
基金
美国国家科学基金会;
关键词
Photocatalysts; Bi2S3/SnS2; heterojunctions; Degradation; Methyl orange; Visible light; HEXAGONAL SNS2 NANOSHEETS; ION-EXCHANGE SYNTHESIS; HIGH-PERFORMANCE; TIN DISULFIDE; SOLVOTHERMAL SYNTHESIS; AZO-DYE; NANOCOMPOSITES; SEMICONDUCTOR; OXIDATION; REDUCTION;
D O I
10.1016/j.jallcom.2016.03.031
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this work, Bi2S3/SnS2 heterojunction photocatalysts were prepared by combining a hydrothermal technique and a facile in situ growth method. The nanocomposites were characterized by X-ray diffraction, scanning electron microscopy, transmission electron microscopy, inductively coupled plasma spectroscopy, X-ray photoelectron spectroscopy, UVeVis diffusion reflectance spectroscopy and room-temperature photoluminescence spectra. Their photocatalytic performances were evaluated by degrading methyl orange (MO) in aqueous solution (50 mg/L) under visible light (lambda > 420 nm) irradiation. It was found that when the mass percentage of Bi2S3 in Bi2S3/SnS2 was 7.95 wt%, the as-prepared Bi2S3/SnS2 nanocomposite showed the best photocatalytic activity for the degradation of MO. The highly improved performance of the Bi2S3/SnS2 nanocomposite was mainly ascribed to the efficient charge separation. (C) 2016 Elsevier B. V. All rights reserved.
引用
收藏
页码:98 / 108
页数:11
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