Crumpled graphene balls as rapid and efficient adsorbents for removal of copper ions

被引:26
作者
Chen, Deqiang [1 ]
Liu, Xiang [1 ]
Nie, Huali [1 ,2 ]
机构
[1] Donghua Univ, Coll Chem Chem Engn & Biotechnol, Shanghai 201620, Peoples R China
[2] Yancheng Polytech Coll, Jiangsu R&D Ctr Ecol Text Engn & Technol, Yancheng 224000, Jiangsu, Peoples R China
关键词
Crumpled graphene balls; Copper ions; Adsorption; Water treatment; HEAVY-METAL IONS; AQUEOUS-SOLUTION; ADSORPTION PROPERTIES; OXIDE; CHITOSAN; NANOPARTICLES; WATER; CU2+; PB(II); CU(II);
D O I
10.1016/j.jcis.2018.06.051
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A novel, three-dimensional (3D), self-supporting material the crumpled graphene ball was developed using an aerosol capillary approach. The resultant crumpled-graphene-ball architecture showed a self-supporting, 3D network microstructure with plenty of ridges and wrinkles. Due to their unique structural characteristics, the 3D balls exhibited a rapid adsorption rate and superior adsorption capacity toward the copper ion (Cu2+). It was noted that the adsorption capacity for Cu2+ reached about 224.56 mg/g within 2 min. A high adsorption capacity, fast adsorption kinetics, excellent regeneration and reusability characteristics, and the ease of materials processing make these crumpled graphene balls ideal candidates for heavy metal ion decontamination in practical application. (C) 2018 Elsevier Inc. All rights reserved.
引用
收藏
页码:46 / 51
页数:6
相关论文
共 48 条
  • [1] Removal of Heavy Metals from Industrial Wastewaters: A Review
    Azimi, Arezoo
    Azari, Ahmad
    Rezakazemi, Mashallah
    Ansarpour, Meisam
    [J]. CHEMBIOENG REVIEWS, 2017, 4 (01): : 37 - 59
  • [2] Efficient techniques for the removal of toxic heavy metals from aquatic environment: A review
    Carolin, C. Femina
    Kumar, P. Senthil
    Saravanan, A.
    Joshiba, G. Janet
    Naushad, Mu.
    [J]. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2017, 5 (03): : 2782 - 2799
  • [3] Graphene oxide functionalized with ethylenediamine triacetic acid for heavy metal adsorption and anti-microbial applications
    Carpio, Isis E. Mejias
    Mangadlao, Joey D.
    Nguyen, Hang N.
    Advincula, Rigoberto C.
    Rodrigues, Debora F.
    [J]. CARBON, 2014, 77 : 289 - 301
  • [4] Comparative adsorption of Cu(II), Zn(II), and Pb(II) ions in aqueous solution on the crosslinked chitosan with epichlorohydrin
    Chen, Arh-Hwang
    Liu, Sheng-Chang
    Chen, Chia-Yuan
    Chen, Chia-Yun
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2008, 154 (1-3) : 184 - 191
  • [5] A phosphorylethanolamine-functionalized super-hydrophilic 3D graphene-based foam filter for water purification
    Chen, Yiying
    Song, Xinhong
    Zhao, Tingting
    Xiao, Yujuan
    Wang, Yiru
    Chen, Xi
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2018, 343 : 298 - 303
  • [6] Tunable assembly of graphene oxide surfactant sheets: wrinkles, overlaps and impacts on thin film properties
    Cote, Laura J.
    Kim, Jaemyung
    Zhang, Zhen
    Sun, Cheng
    Huang, Jiaxing
    [J]. SOFT MATTER, 2010, 6 (24) : 6096 - 6101
  • [7] Developing stretchable and graphene-oxide-based hydrogel for the removal of organic pollutants and metal ions
    Dong, Chencheng
    Lu, Jie
    Qiu, Bocheng
    Shen, Bin
    Xing, Mingyang
    Zhang, Jinlong
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2018, 222 : 146 - 156
  • [8] Self-dispersed crumpled graphene balls in oil for friction and wear reduction
    Dou, Xuan
    Koltonow, Andrew R.
    He, Xingliang
    Jang, Hee Dong
    Wang, Qian
    Chung, Yip-Wah
    Huang, Jiaxing
    [J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2016, 113 (06) : 1528 - 1533
  • [9] Graphene oxides for removal of heavy and precious metals from wastewater
    Duru, Ilayda
    Ege, Duygu
    Kamali, Ali Reza
    [J]. JOURNAL OF MATERIALS SCIENCE, 2016, 51 (13) : 6097 - 6116
  • [10] Interaction of stevensite with Cd2+ and Pb2+ in aqueous dispersions
    El Mouzdahir, Y.
    Elmchaouri, A.
    Mahboub, R.
    ElAnssari, A.
    Gil, A.
    Korili, S. A.
    Vicente, M. A.
    [J]. APPLIED CLAY SCIENCE, 2007, 35 (1-2) : 47 - 58