Preparation of LaMnO3/graphene thin films and their photocatalytic activity

被引：41

作者：

Hu Jie ^{[1
,2
]}

Men Jie ^{[1
]}

Ma Jiahua ^{[1
]}

Huang Hao ^{[2
]}

机构：

[1] Yanshan Univ, Dept Environm & Chem, Hebei Key Lab Appl Chem, Qinhuangdao 066004, Peoples R China

[2] Yanshan Univ, State Key Lab Metastable Mat Sci & Technol, Qinhuangdao 066004, Peoples R China

来源：

JOURNAL OF RARE EARTHS | 2014年 / 32卷 / 12期

基金：

中国国家自然科学基金;

关键词：

perovskite; graphene; film; photocatalysts; rare earths; COMPOSITES; BI2WO6; DEGRADATION; DYE; AG;

D O I：

10.1016/S1002-0721(14)60193-9

中图分类号：

O69 [应用化学];

学科分类号：

081704 ;

摘要：

A novel photocatalyst of LaMnO3/graphene thin films with the perovskite-type was synthesized by sol-gel process assisted with spin-coating methods on glass substrates. The prepared samples were characterized by scanning electron microscopy (SEM), transmission electron microscopy (TEM), X-ray diffraction (XRD), Brumauer-Emmett-Teller (BET) surface area analyzer, X-ray photoelectron spectroscopy (XPS) and UV-vis diffuse reflectance spectroscopy. Results showed that after the introduction of graphene, the perovskite structure was unchanged and the size of LaMnO3 particles was about 22 nm, which uniformed growth in graphene sheet. Determination of contact angle indicated that the contact angle of glass substrate decreased and the hydrophilicity improved after treating with H2SO4 and APTES. The UV-Vis photocatalytic activity of the photocatalysts was evaluated by the degradation of diamine green B. LaMnO3/graphene thin films had better photocatalytic ability than LaMnO3 and TiO2 films. The obtained k was 0.5627 and 0.3441 h(-1) corresponding to LaMnO3/graphene films and TiO2 films, respectively.

引用

页码：1126 / 1134

页数：9

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