Stable bright perovskite nanoparticle thin porous films for color enhancement in modern liquid crystal displays

被引:18
作者
Gao, Yiyang [1 ,2 ]
Prodanov, Maksym F. [1 ,2 ]
Kang, Chengbin [1 ,2 ]
Vashchenko, Valerii V. [1 ,2 ]
Gupta, Swadesh K. [1 ,2 ]
Chan, Christopher C. S. [3 ]
Wong, Kam Sing [3 ]
Srivastava, Abhishek K. [1 ,2 ]
机构
[1] Hong Kong Univ Sci & Technol, State Key Lab Adv Displays & Optoelect Technol, Hong Kong, Peoples R China
[2] Hong Kong Univ Sci & Technol, Ctr Display Res, Dept Elect & Comp Engn, Hong Kong, Peoples R China
[3] Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Peoples R China
关键词
ORGANIC-INORGANIC PEROVSKITE; LEAD HALIDE PEROVSKITES; LIGHT-EMITTING-DIODES; QUANTUM DOTS; CSPBX3; X; NANOCRYSTALS; CSPBBR3; STABILITY; PHOTOLUMINESCENCE; LUMINESCENCE;
D O I
10.1039/d0nr07313j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Cesium-lead halide perovskite nanoparticles are a promising class of luminescent materials for color and efficient displays. However, material stability is the key issue to solve before we can use these materials in modern displays. Encapsulation is one of the most efficient methods that can markedly improve the stability of perovskite nanoparticles against moisture, heat, oxygen, and light. Thus, we urgently need a low-cost, reliable, and device-compatible encapsulation method for the integration of nanomaterials into display devices. Here, we propose a facile encapsulation method to stabilize perovskite nanoparticles in thin polymer porous films. Using porous polymer films, we achieved good photoluminescence stability in the harsh environment of high temperature, high humidity and strong UV illumination. The good UV stability benefitted from the unique optical properties of the porous film. Besides, we observed photoluminescence enhancement of CsPbBr3 nanoparticle films in a high humidity environment. The stable CsPbBr3 nanoparticle thin porous film provides high brightness (236 nits) and great color enhancement for LCDs and is characterized by simple fabrication with easy scalability, thus it is very suitable for modern LCDs.
引用
收藏
页码:6400 / 6409
页数:10
相关论文
共 58 条
[1]   Tuning the Optical Properties of Cesium Lead Halide Perovskite Nanocrystals by Anion Exchange Reactions [J].
Akkerman, Quinten A. ;
D'Innocenzo, Valerio ;
Accornero, Sara ;
Scarpellini, Alice ;
Petrozza, Annamaria ;
Prato, Mirko ;
Manna, Liberato .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (32) :10276-10281
[2]   Colloidal metal halide perovskite nanocrystals: synthesis, characterization, and applications [J].
Bai, Sai ;
Yuan, Zhongcheng ;
Gao, Feng .
JOURNAL OF MATERIALS CHEMISTRY C, 2016, 4 (18) :3898-3904
[3]   The Evolution of Quantum Confinement in CsPbBr3 Perovskite Nanocrystals [J].
Butkus, Justinas ;
Vashishtha, Parth ;
Chen, Kai ;
Gallaher, Joseph K. ;
Prasad, Shyamal K. K. ;
Metin, Dani Z. ;
Laufersky, Geoffry ;
Gaston, Nicola ;
Halpert, Jonathan E. ;
Hodgkiss, Justin M. .
CHEMISTRY OF MATERIALS, 2017, 29 (08) :3644-3652
[4]   Size-controllable and stable organometallic halide perovskite quantum dots/polymer films [J].
Cha, Wonhee ;
Kim, Hae-Jin ;
Lee, Songhee ;
Kim, Jiwon .
JOURNAL OF MATERIALS CHEMISTRY C, 2017, 5 (27) :6667-6671
[5]   In Situ Fabricated Perovskite Nanocrystals: A Revolution in Optical Materials [J].
Chang, Shuai ;
Bai, Zelong ;
Zhong, Haizheng .
ADVANCED OPTICAL MATERIALS, 2018, 6 (18)
[6]   Recent Advances on Quantum-Dot-Enhanced Liquid-Crystal Displays [J].
Chen, Haiwei ;
He, Juan ;
Wu, Shin-Tson .
IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, 2017, 23 (05)
[7]   Light Illumination Induced Photoluminescence Enhancement and Quenching in Lead Halide Perovskite [J].
Chen, Sheng ;
Wen, Xiaoming ;
Huang, Shujuan ;
Huang, Fuzhi ;
Cheng, Yi-Bing ;
Green, Martin ;
Ho-Baillie, Anita .
SOLAR RRL, 2017, 1 (01)
[8]   A Confined Fabrication of Perovskite Quantum Dots in Oriented MOF Thin Film [J].
Chen, Zheng ;
Gu, Zhi-Gang ;
Fu, Wen-Qiang ;
Wang, Fei ;
Zhang, Jian .
ACS APPLIED MATERIALS & INTERFACES, 2016, 8 (42) :28737-28742
[9]   Highly Dynamic Ligand Binding and Light Absorption Coefficient of Cesium Lead Bromide Perovskite Nanocrystals [J].
De Roo, Jonathan ;
Ibanez, Maria ;
Geiregat, Pieter ;
Nedelcu, Georgian ;
Walravens, Willem ;
Maes, Jorick ;
Martins, Jose C. ;
Van Driessche, Isabel ;
Koyalenko, Maksym V. ;
Hens, Zeger .
ACS NANO, 2016, 10 (02) :2071-2081
[10]   Dual effect of humidity on cesium lead bromide: enhancement and degradation of perovskite films [J].
Di Girolamo, Diego ;
Dar, M. Ibrahim ;
Dini, Danilo ;
Gontrani, Lorenzo ;
Caminiti, Ruggero ;
Mattoni, Alessandro ;
Graetzel, Michael ;
Meloni, Simone .
JOURNAL OF MATERIALS CHEMISTRY A, 2019, 7 (19) :12292-12302