Structural arrest transitions in fluids described by two Yukawa potentials

被引:0
|
作者
Wu, JL
Liu, Y
Chen, WR
Cao, JS
Chen, SH [1 ]
机构
[1] MIT, Dept Nucl Engn, Cambridge, MA 02139 USA
[2] MIT, Dept Chem, Cambridge, MA 02139 USA
来源
PHYSICAL REVIEW E | 2004年 / 70卷 / 05期
关键词
D O I
暂无
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We study a model colloidal system where particles interact via short-range attractive and long-range repulsive Yukawa potentials. Using the structure factor calculated from the mean-spherical approximation as the input, the kinetic phase diagrams as functions of the attraction depth and the volume fraction are obtained by calculating the Debye-Waller factors in the framework of the mode-coupling theory for three different heights of the repulsive barrier. The glass-glass reentrance phenomenon in the attractive colloidal case is also observed in the presence of the long-range repulsive barrier, which results in the lower and upper glass regimes. Competition between the short-range attraction and the long-range repulsion gives rise to new regimes associated with clusters such as "static cluster glass" and "dynamic cluster glass," which appear in the lower glass regime. Along the liquid-glass transition line between the liquid regime and the lower glass regime, crossover points separating different glass states are identified.
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页数:4
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