Optical evidence of metal-insulator phase transition in A1C60

被引:2
作者
Bommeli, F [1 ]
Degiorgi, L
Wachter, P
Forro, L
机构
[1] ETH Zurich, Festkorperphys Lab, CH-8093 Zurich, Switzerland
[2] EPF Lausanne, IGA Dept Phys, Lab Phys Solides Semicristallins, CH-1015 Lausanne, Switzerland
关键词
D O I
10.1016/S0022-3697(97)00068-1
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We have investigated the complete electrodynamic response of the newly discovered alkali fulleride linear polymers A(1)C(60) We find clear evidence for a metal-insulator phase transition al low temperatures in Rb1C60 and Cs1C60, while the K-compound remains metallic at all temperatures. The possibility of a broken symmetry ground state due to the formation of a spin-density-wave for the Rb and Cs compound, as suggested by the magnetic properties, is discussed. (C) 1997 Elsevier Science Ltd.
引用
收藏
页码:1797 / 1802
页数:6
相关论文
共 14 条
[1]   METALLIC CONDUCTIVITY AND METAL-INSULATOR-TRANSITION IN (AC(60))(N) (A=K, RB, AND CS) LINEAR POLYMER FULLERIDES [J].
BOMMELI, F ;
DEGIORGI, L ;
WACHTER, P ;
LEGEZA, O ;
JANOSSY, A ;
OSZLANYI, G ;
CHAUVET, O ;
FORRO, L .
PHYSICAL REVIEW B, 1995, 51 (20) :14794-14797
[2]   QUASI-ONE-DIMENSIONAL ELECTRONIC-STRUCTURE IN ORTHORHOMBIC RBC60 [J].
CHAUVET, O ;
OSZLANYI, G ;
FORRO, L ;
STEPHENS, PW ;
TEGZE, M ;
FAIGEL, G ;
JANOSSY, A .
PHYSICAL REVIEW LETTERS, 1994, 72 (17) :2721-2724
[3]   OPTICAL-PROPERTIES OF THE ALKALI-METAL-DOPED SUPERCONDUCTING FULLERENES - K3C60 AND RB3C60 [J].
DEGIORGI, L ;
NICOL, EJ ;
KLEIN, O ;
GRUNER, G ;
WACHTER, P ;
HUANG, SM ;
WILEY, J ;
KANER, RB .
PHYSICAL REVIEW B, 1994, 49 (10) :7012-7025
[4]   THE DYNAMICS OF SPIN-DENSITY WAVES [J].
GRUNER, G .
REVIEWS OF MODERN PHYSICS, 1994, 66 (01) :1-24
[5]   CONDUCTION ELECTRON-SPIN-RESONANCE IN RB3C60 [J].
JANOSSY, A ;
CHAUVET, O ;
PEKKER, S ;
COOPER, JR ;
FORRO, L .
PHYSICAL REVIEW LETTERS, 1993, 71 (07) :1091-1094
[6]   INSULATING AND CONDUCTING PHASES OF RBC60 [J].
MARTIN, MC ;
KOLLER, D ;
DU, XQ ;
STEPHENS, PW ;
MIHALY, L .
PHYSICAL REVIEW B, 1994, 49 (15) :10818-10821
[7]   ORTHORHOMBIC A(1)C60 - A CONDUCTING LINEAR ALKALI FULLERIDE POLYMER [J].
PEKKER, S ;
FORRO, L ;
MIHALY, L ;
JANOSSY, A .
SOLID STATE COMMUNICATIONS, 1994, 90 (06) :349-352
[8]   EQUILIBRIUM PHASES IN K-DOPED AND RB-DOPED C(60) FROM IN-SITU INFRARED REFLECTIVITY MEASUREMENTS [J].
PICHLER, T ;
WINKLER, R ;
KUZMANY, H .
PHYSICAL REVIEW B, 1994, 49 (22) :15879-15889
[9]  
POIRER DM, 1993, PHYS REV B, V47, P10867
[10]   KC60 FULLERIDE PHASE FORMATION - AN X-RAY PHOTOEMISSION-STUDY [J].
POIRIER, DM ;
WEAVER, JH .
PHYSICAL REVIEW B, 1993, 47 (16) :10959-10962