Characterization, seasonal variation, source apportionment and health risk assessment of black carbon over an urban region of East India

被引:58
作者
Ambade, Balram [1 ]
Sankar, Tapan Kumar [1 ]
Panicker, A. S. [2 ]
Gautam, Alok Sagar [3 ]
Gautam, Sneha [4 ]
机构
[1] Natl Inst Technol, Dept Chem, Jamshedpur 831014, Jharkhand, India
[2] Govt India, MoES, Indian Inst Trop Meteorol, Pune, Maharashtra, India
[3] Hemvati Nandan Bahuguna Garhwal Univ, Dept Phys, Garhwal 246174, Uttarakhand, India
[4] Karunya Inst Technol & Sci, Coimbatore 641114, Tamil Nadu, India
关键词
Black carbon; Aethalometer; PM2; 5; Backward trajectory; Health risk assessment; AIR-POLLUTION; AEROSOL EMISSIONS; ELEMENTAL CARBON; PARTICLES; EXPOSURE; CLIMATE; AETHALOMETER; COMBUSTION; ABSORPTION; IMPACTS;
D O I
10.1016/j.uclim.2021.100896
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Black carbon (BC) is produced due to the incomplete combustion of fossil fuels and rapidly accelerates the globe. The study of the source apportionment exploration of BC is inaccurate due to lacking observational limitations and uncertainties in emission inventories. In the present work, we measured BC mass concentrations using a 7-wavelength Aethalometer (AE-33). In this study, BC mass concentration was ranging from 2 to 13.43 mu gm- 3 and was minimum during monsoon (3.23 +/- 0.38 mu gm-3) and maximum in the winter season (11.68 +/- 2.55 mu gm- 3). The annual mean BC mass concentration and PM2.5 were reported as 6.60 +/- 3.50 mu gm- 3 and 119.07 +/- 43.44 mu gm3, respectively. In overall study, the BC aerosol was contributing 6.92% (winter), 5.09% (summer), 3.79% (monsoon) and 5.25% (post-monsoon) to the total mass concentration of PM2.5. Backward Trajectories have shown that the airborne particulate matter comes from different directions in different seasons. Correlation analysis has found a strong relationship between BC and PM2.5 (r = 0.89, r2 = 0.80). However, an inverse relationship was noticed between BC and temperature(r = -0.92), wind speed (r = -0.61), precipitation (r = -0.60) and humidity (r = -0.52) during the observational period. Apart from describing BC's atmospheric impacts, the health risk assessment of BC during various seasons over Jamshedpur city is also illustrated in detail.
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页数:12
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