Rare earth-doped LiLuF4 microcrystalline for high-efficiency scintillation and X-ray imaging applications

被引:6
作者
Zheng, Yi [1 ,2 ]
Xu, Hui [3 ]
Xu, XieMing [1 ,2 ]
Xu, LiuWei [1 ]
Wang, ShuaiHua [1 ]
Wu, ShaoFan [1 ]
机构
[1] Chinese Acad Sci, Fujian Inst Res Struct Matter, Key Lab Optoelect Mat Chem & Phys, Fuzhou 350002, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] CASTECH Inc, Fuzhou 350003, Peoples R China
基金
中国国家自然科学基金;
关键词
Microcrystalline; X-ray imaging; Light output; Spatial resolution capability; Flexible scintillation film; SINGLE-CRYSTAL; PHOTOIONIZATION; DETECTORS;
D O I
10.1016/j.jallcom.2022.164778
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Scintillators play a vital role in high-energy physics, medical imaging, security inspection, etc. Here, we designed and prepared a highly efficient scintillator of Ce,Tb-codoped LiLuF4, which was synthesized by a hydrothermal method using low-cost raw materials. The microcrystalline scintillator exhibits the strong luminescence of rare earth ion, which has a characteristic green fluorescence emission with a quantum yield of 71.59%. This material has a strong X-ray response, superior light output (16,509 ph/MeV), excellent ray cut-off capability and absolute stability. Based on micron-level powdered compounds, we used direct coating to manufacture a scintillation film with a size of 5.5 cm x 8.0 cm for X-ray imaging testing. The imaging test shows that the highly stable scintillation film not only has a spatial resolution capability of more than 10.0 LP/mm but also has great potential to be prepared as a flexible scintillator, which exhibited excellent performance as an potential scintillation detection material. (C)& nbsp;2022 Published by Elsevier B.V.
引用
收藏
页数:7
相关论文
共 42 条
  • [21] Pei XJ, 2005, SPECTROSC SPECT ANAL, V25, P819
  • [22] Physcial Measurement Laboratory, 2022, PHOT CROSS SECT DAT
  • [23] Polymer Composites Entrapped Ce-Doped LiYF4 Microcrystals for High-Sensitivity X-ray Scintillation and Imaging
    Qiu, Zhihua
    Wang, Shuaihua
    Wang, Wenqian
    Wu, Shaofan
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2020, 12 (26) : 29835 - 29843
  • [24] Crystal structure, optical spectroscopy and energy transfer properties in NaZnPO4:Ce3+, Tb3+phosphors for UV-based LEDs
    Saidi, K.
    Dammak, M.
    [J]. RSC ADVANCES, 2020, 10 (37) : 21867 - 21875
  • [25] STUDY OF ORGANIC SCINTILLATORS
    SANGSTER, RC
    IRVINE, JW
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1956, 24 (04) : 670 - 715
  • [26] Mesoscopic fast ion conduction in nanometre-scale planar heterostructures
    Sata, N
    Eberman, K
    Eberl, K
    Maier, J
    [J]. NATURE, 2000, 408 (6815) : 946 - 949
  • [27] Sedov V., ACS APPL NANO MATER
  • [28] Size-controllable luminescent single crystal CaF2 nanocubes
    Sun, XM
    Li, YD
    [J]. CHEMICAL COMMUNICATIONS, 2003, (14) : 1768 - 1769
  • [29] CERIUM-ACTIVATED GD2SIO5 SINGLE-CRYSTAL SCINTILLATOR
    TAKAGI, K
    FUKAZAWA, T
    [J]. APPLIED PHYSICS LETTERS, 1983, 42 (01) : 43 - 45
  • [30] Concentration dependence of the light yield and energy resolution of NaI:Tl and CsI:Tl crystals excited by gamma, soft X-rays and alpha particles
    Trefilova, LN
    Kudin, AM
    Kovaleva, LV
    Zaslavsky, BG
    Zosim, DI
    Bondarenko, SK
    [J]. NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2002, 486 (1-2) : 474 - 481