High-performance Al2O3-YAG:Ce composite ceramic phosphors for miniaturization of high-brightness white light-emitting diodes

被引:39
作者
Zhao, Huanyu [1 ]
Li, Zhi [2 ]
Zhang, Mengwen [1 ]
Li, Jinsheng [1 ]
Wu, Minbo [1 ]
Li, Xiaodong [1 ]
Chen, Jialin [3 ]
Xie, Ming [3 ]
Li, Junpeng [3 ]
Sun, Xudong [1 ,2 ]
机构
[1] Northeastern Univ, Sch Mat Sci & Engn, Key Lab Anisotropy & Texture Mat, Minist Educ, Shenyang 110819, Liaoning, Peoples R China
[2] Dalian Univ, Coll Environm & Chem Engn, Liaoning Engn Lab Special Opt Funct Crystals, Dalian 116622, Peoples R China
[3] Kunming Inst Precious Met, State Key Lab Adv Technol Comprehens Utilizat Pla, Kunming 650106, Yunnan, Peoples R China
基金
中国国家自然科学基金;
关键词
Thermal conductivity; Al2O3-YAG:Ce; Ceramic phosphor; WLED; HIGH-POWER LEDS; THERMAL-CONDUCTIVITY; TRANSPARENT CERAMICS; MICROSTRUCTURE; EFFICIENCY; STABILITY; LUMINESCENCE; CONVERTER; EXPANSION; Y3AL5O12;
D O I
10.1016/j.ceramint.2019.09.017
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The miniaturization of high-brightness white light-emitting diodes (WLEDs) is limited by the low thermal performance of phosphors. In this study, the microstructure, optical properties, and thermal performance of Al2O3-Y3Al5O12:Ce3+ (Al2O3-YAG:Ce) composite ceramics fabricated by hot pressing were investigated. By promoting the growth of Al2O3 grains while maintaining a high composite density, thermal performance of the composite ceramics was significantly increased. The thermal conductivity of a Al2O3-40-vol% YAG:Ce ceramic reached 21.8 W/m/K, which is close to the theoretical value. In addition, this composite ceramic exhibited the highest energy efficiency. After packaging with a high-power LED chip with dimensions of 1 mm x 1 mm, a high luminous flux of 639 1m was generated, while the reduction in output power at 250 degrees C was as low as 6%. This indicated excellent high-temperature stability and potential for applications in solid-state lighting.
引用
收藏
页码:653 / 662
页数:10
相关论文
共 47 条
[41]   Thermal-Stability Comparison of Glass- and Silicone-Based High-Power Phosphor-Converted White-Light-Emitting Diodes Under Thermal Aging [J].
Tsai, Chun-Chin ;
Cheng, Wei-Chih ;
Chang, Jin-Kai ;
Huang, Shun-Yuan ;
Liou, Jyun-Sian ;
Chen, Gi-Hung ;
Huang, Yi-Chung ;
Wang, Jau-Sheng ;
Cheng, Wood-Hi .
IEEE TRANSACTIONS ON DEVICE AND MATERIALS RELIABILITY, 2014, 14 (01) :4-8
[42]   YAG: Ce3+,Mn2+ transparent ceramics prepared by gel-casting for warm white LEDs [J].
Wang, Bin ;
Ling, Junrong ;
Zhou, Youfu ;
Xu, Wentao ;
Lin, He ;
Lu, Shuai ;
Qin, Zixuan ;
Hong, Maochun .
JOURNAL OF LUMINESCENCE, 2019, 213 :421-426
[43]   In-situ preparation of MgFe2O4-GO nanocomposite and its enhanced catalytic reactivity on decomposition of AP and RDX [J].
Wang, Weimin ;
Liu, Bo ;
Xu, Kangzhen ;
Zu, Yanqing ;
Song, Jirong ;
Zhao, Fengqi .
CERAMICS INTERNATIONAL, 2018, 44 (15) :19016-19020
[44]   Four-wave mixing microscopy of nanostructures [J].
Wang, Yong ;
Lin, Chia-Yu ;
Nikolaenko, Alexei ;
Raghunathan, Varun ;
Potma, Eric O. .
ADVANCES IN OPTICS AND PHOTONICS, 2011, 3 (01) :1-52
[45]   Al2O3-YAG:Ce composite ceramics for high-brightness lighting [J].
Xu, M. ;
Chang, J. ;
Wang, J. ;
Wu, C. ;
Hu, F. .
OPTICS EXPRESS, 2019, 27 (02) :872-885
[46]   A new-generation color converter for high-power white LED: transparent Ce3+:YAG phosphor-in-glass [J].
Zhang, Rui ;
Lin, Hang ;
Yu, Yunlong ;
Chen, Daqin ;
Xu, Ju ;
Wang, Yuansheng .
LASER & PHOTONICS REVIEWS, 2014, 8 (01) :158-164
[47]   Pore-existing Lu3Al5O12:Ce ceramic phosphor: An efficient green color converter for laser light source [J].
Zhang, Yunli ;
Hu, Song ;
Wang, Zhengjuan ;
Zhou, Guohong ;
Wang, Shiwei .
JOURNAL OF LUMINESCENCE, 2018, 197 :331-334