Transport Properties and Finite Size Effects in β-Ga2O3 Thin Films

被引:11
作者
Ahrling, Robin [1 ]
Boy, Johannes [1 ]
Handwerg, Martin [1 ]
Chiatti, Olivio [1 ]
Mitdank, Ruediger [1 ]
Wagner, Guenter [2 ]
Galazka, Zbigniew [2 ]
Fischer, Saskia F. [1 ]
机构
[1] Humboldt Univ, Novel Mat Grp, Newtonstr 15, D-12489 Berlin, Germany
[2] Leibniz Inst Crystal Growth, Max Born Str 2, D-12489 Berlin, Germany
关键词
MEAN FREE-PATH; ELECTRICAL-PROPERTIES; SINGLE-CRYSTALS; ELECTRONS; GROWTH; LAYERS;
D O I
10.1038/s41598-019-49238-2
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Thin films of the wide band gap semiconductor beta-Ga2O3 have a high potential for applications in transparent electronics and high power devices. However, the role of interfaces remains to be explored. Here, we report on fundamental limits of transport properties in thin films. The conductivities, Hall densities and mobilities in thin homoepitaxially MOVPE grown (100)-orientated beta-Ga2O3 films were measured as a function of temperature and film thickness. At room temperature, the electron mobilities ((115 +/- 10)cm(2)/Vs) in thicker films (>150 nm) are comparable to the best of bulk. However, the mobility is strongly reduced by more than two orders of magnitude with decreasing film thickness ((5.5 +/- 0.5) cm(2)/Vs for a 28 nm thin film). We find that the commonly applied classical Fuchs-Sondheimer model does not explain sufficiently the contribution of electron scattering at the film surfaces. Instead, by applying an electron wave model by Bergmann, a contribution to the mobility suppression due to the large de Broglie wavelength in beta-Ga2O3 is proposed as a limiting quantum mechanical size effect.
引用
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页数:9
相关论文
共 36 条
[1]   Shear-induced mechanical failure of β-Ga2O3 from quantum mechanics simulations [J].
An, Qi ;
Li, Guodong .
PHYSICAL REVIEW B, 2017, 96 (14)
[2]   CONDUCTION IN THIN SEMICONDUCTOR FILMS [J].
ANDERSON, JC .
ADVANCES IN PHYSICS, 1970, 19 (79) :311-&
[3]   Si- and Sn-Doped Homoepitaxial β-Ga2O3 Layers Grown by MOVPE on (010)-Oriented Substrates [J].
Baldini, Michele ;
Albrecht, Martin ;
Fiedler, Andreas ;
Irmscher, Klaus ;
Schewski, Robert ;
Wagner, Guenter .
ECS JOURNAL OF SOLID STATE SCIENCE AND TECHNOLOGY, 2017, 6 (02) :Q3040-Q3044
[4]   Conductance of a perfect thin film with diffuse surface scattering [J].
Bergmann, G .
PHYSICAL REVIEW LETTERS, 2005, 94 (10)
[5]   High-Resolution ac Measurements of the Hall Effect in Organic Field-Effect Transistors [J].
Chen, Y. ;
Yi, H. T. ;
Podzorov, V. .
PHYSICAL REVIEW APPLIED, 2016, 5 (03)
[6]   Influence of incoherent twin boundaries on the electrical properties of β-Ga2O3 layers homoepitaxially grown by metal-organic vapor phase epitaxy [J].
Fiedler, A. ;
Schewski, R. ;
Baldini, M. ;
Galazka, Z. ;
Wagner, G. ;
Albrecht, M. ;
Irmscher, K. .
JOURNAL OF APPLIED PHYSICS, 2017, 122 (16)
[7]   Transparent conducting oxides for photovoltaics [J].
Fortunato, Elvira ;
Ginley, David ;
Hosono, Hideo ;
Paine, David C. .
MRS BULLETIN, 2007, 32 (03) :242-247
[8]   The conductivity of thin metallic films according to the electron theory of metals [J].
Fuchs, K .
PROCEEDINGS OF THE CAMBRIDGE PHILOSOPHICAL SOCIETY, 1938, 34 :100-108
[9]   Czochralski growth and characterization of β-Ga2O3 single crystals [J].
Galazka, Z. ;
Uecker, R. ;
Irmscher, K. ;
Albrecht, M. ;
Klimm, D. ;
Pietsch, M. ;
Bruetzam, M. ;
Bertram, R. ;
Ganschow, S. ;
Fornari, R. .
CRYSTAL RESEARCH AND TECHNOLOGY, 2010, 45 (12) :1229-1236
[10]   Scaling-Up of Bulk β-Ga2O3 Single Crystals by the Czochralski Method [J].
Galazka, Zbigniew ;
Uecker, Reinhard ;
Klimm, Detlef ;
Irmscher, Klaus ;
Naumann, Martin ;
Pietsch, Mike ;
Kwasniewski, Albert ;
Bertram, Rainer ;
Ganschow, Steffen ;
Bickermann, Matthias .
ECS JOURNAL OF SOLID STATE SCIENCE AND TECHNOLOGY, 2017, 6 (02) :Q3007-Q3011