Gabuda's model of averaging local magnetic fields in solid-state NMR. The mobility of atoms and molecules

被引:7
|
作者
Kozlova, S. G. [1 ]
Sergeev, N. A. [2 ]
Buznik, V. M. [3 ,4 ]
机构
[1] Russian Acad Sci, Nikolaev Inst Inorgan Chem, Siberian Branch, Novosibirsk, Russia
[2] Univ Szczecin, Inst Phys, PL-70453 Szczecin, Poland
[3] All Russian Sci Res Inst Aviat Mat, Moscow, Russia
[4] Tomsk Natl Res State Univ, Tomsk, Russia
关键词
NMR; mobility of atoms and molecules; solids; minerals; sorbents; hydrated proteins; WATER-MOLECULES; GUEST SUBLATTICE; STRUCTURAL TRANSFORMATIONS; SPONTANEOUS POLARIZATION; PHASE-TRANSITION; ZEOLITE WATER; SQUARIC ACID; BOUND WATER; RESONANCE; DIFFUSION;
D O I
10.1134/S0022476616020013
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
The review presents the main results of the studies of Prof. S. P. Gabuda, which were devoted to the NMR investigation of the mobility of atoms and molecules. The basic principles of his model for averaging local magnetic fields under the conditions of atomic and molecular mobility are outlined. This model provides a relationship between the parameters of these fields with the structural features of the mobility of atoms and molecules and intermolecular interactions. Ionic and molecular crystals, zeolites, molecular sieves, hydrated proteins, and so on are considered. Phase transitions in guest subsystems, effects of dynamic disordering and correlated electron motion on the mobility of atoms and molecules and their location are discussed.
引用
收藏
页码:213 / 237
页数:25
相关论文
共 48 条
  • [21] Frequency-swept solid-state 33S NMR of an organosulfur compound in an extremely low magnetic field
    Yamada, Kazuhiko
    Aoki, Daisuke
    Kitagawa, Kentaro
    Takata, Toshikazu
    CHEMICAL PHYSICS LETTERS, 2015, 630 : 86 - 90
  • [22] Local environments and dynamics of hydrogen atoms in protonated forms of ion-exchangeable layered perovskites estimated by solid-state 1H NMR
    Tani, Shinsuke
    Komori, Yoshihiko
    Hayashi, Shigenobu
    Sugahara, Yoshiyuki
    JOURNAL OF SOLID STATE CHEMISTRY, 2006, 179 (11) : 3357 - 3364
  • [23] Effect of Dehydration on the Local Structure of Framework Aluminum Atoms in Mixed Linker MIL-53(Al) Materials Studied by Solid-State NMR Spectroscopy
    Jiang, Yijiao
    Huang, Jun
    Marx, Stefan
    Kleist, Wolfgang
    Hunger, Michael
    Baiker, Alfons
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2010, 1 (19): : 2886 - 2890
  • [24] Biphenyl bicelle disks align perpendicular to magnetic fields on large temperature scales: A study combining synthesis, solid-state NMR, TEM, and SAXS
    Loudet, Cecile
    Manet, Sabine
    Gineste, Stephane
    Oda, Reiko
    Achard, Marie-France
    Dufourc, Erick J.
    BIOPHYSICAL JOURNAL, 2007, 92 (11) : 3949 - 3959
  • [25] Influence of hidden halogen mobility on local structure of CsSn(Cl1-xBrx)3 mixed-halide perovskites by solid-state NMR
    Karmakar, Abhoy
    Bhattacharya, Amit
    Sarkar, Diganta
    Bernard, Guy M.
    Mar, Arthur
    Michaelis, Vladimir K.
    CHEMICAL SCIENCE, 2021, 12 (09) : 3253 - 3263
  • [26] BDPA-Nitroxide Biradicals Tailored for Efficient Dynamic Nuclear Polarization Enhanced Solid-State NMR at Magnetic Fields up to 21.1 T
    Wisser, Dorothea
    Karthikeyan, Ganesan
    Lund, Alicia
    Casano, Gilles
    Karoui, Hakim
    Yulikov, Maxim
    Menzildjian, Georges
    Pinon, Arthur C.
    Purea, Armin
    Engelke, Frank
    Chaudhari, Sachin R.
    Kubicki, Dominik
    Rossini, Aaron J.
    Moroz, Ilia B.
    Gajan, David
    Coperet, Christophe
    Jeschke, Gunnar
    Lelli, Moreno
    Emsley, Lyndon
    Lesage, Anne
    Ouari, Olivier
    JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2018, 140 (41) : 13340 - 13349
  • [27] A natural abundance 33S solid-state NMR study of layered transition metal disulfides at ultrahigh magnetic field
    Sutrisno, Andre
    Terskikh, Victor V.
    Huang, Yining
    CHEMICAL COMMUNICATIONS, 2009, (02) : 186 - 188
  • [28] Carbon-13 solid-state NMR studies on synthetic model compounds of [4Fe-4S] clusters in the 2+ state
    Crozet, M
    Chaussade, M
    Bardet, M
    Emsley, L
    Lamotte, B
    Mouesca, JM
    JOURNAL OF PHYSICAL CHEMISTRY A, 2000, 104 (44): : 9990 - 10000
  • [29] Mechanical behaviour of inorganic solid-state batteries: can we model the ionic mobility in the electrolyte with Nernst-Einstein's relation?
    Pang, Mei-Chin
    Marinescu, Monica
    Wang, Huizhi
    Offer, Gregory
    PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2021, 23 (48) : 27159 - 27170
  • [30] Local conformation of serine residues in a silk model peptide, (Ala–Gly–Ser–Gly–Ala–Gly)5, studied with solid-state NMR:REDOR
    Yu Suzuki
    Tetsuo Asakura
    Polymer Journal, 2010, 42 : 354 - 356