Shining Light on Transition-Metal Oxides: Unveiling the Hidden Fermi Liquid

被引:38
作者
Deng, Xiaoyu [1 ]
Sternbach, Aaron [2 ]
Haule, Kristjan [1 ]
Basov, D. N. [2 ]
Kotliar, Gabriel [1 ]
机构
[1] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA
[2] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA
基金
美国国家科学基金会;
关键词
ELECTRONIC-STRUCTURE CALCULATIONS; OPTICAL CONDUCTIVITY; MOTT; BEHAVIOR; UNIVERSALITY; PHASE; LIMIT; V2O3; HEAT;
D O I
10.1103/PhysRevLett.113.246404
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We use low energy optical spectroscopy and first principles local density approximation plus dynamical mean field theory calculations to test the hypothesis that the anomalous transport properties of strongly correlated metals originate in the strong temperature dependence of their underlying resilient quasiparticles. We express the resistivity in terms of an effective plasma frequency. omega(p)* and an effective scattering rate 1/tau(*)(tr). We show that in the archetypal correlated material V-2 O-3, omega(p)* increases with increasing temperature, while the plasma frequency from the partial sum rule exhibits the opposite trend. 1/tau(*)(tr) has a more pronounced temperature dependence than the scattering rate obtained from the extended Drude analysis. The theoretical calculations of these quantities are in quantitative agreement with experiment. We conjecture that these are robust properties of all strongly correlated metals, and test the conjecture by carrying out a similar analysis on thin film NdNiO3 on a LaAlO3 substrate.
引用
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页数:6
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