Interlayer exciton laser of extended spatial coherence in atomically thin heterostructures

被引:189
作者
Paik, Eunice Y. [1 ]
Zhang, Long [1 ]
Burg, G. William [2 ]
Gogna, Rahul [3 ]
Tutuc, Emanuel [2 ]
Deng, Hui [1 ]
机构
[1] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA
[2] Univ Texas Austin, Dept Elect & Comp Engn, Microelect Res Ctr, Austin, TX 78712 USA
[3] Univ Michigan, Appl Phys Program, Ann Arbor, MI 48109 USA
关键词
D O I
10.1038/s41586-019-1779-x
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Two-dimensional semiconductors have emerged as a new class of materials for nanophotonics owing to their strong exciton-photon interaction(1,2) and their ability to be engineered and integrated into devices(3). Here we take advantage of these properties to engineer an efficient lasing medium based on direct-bandgap interlayer excitons in rotationally aligned atomically thin heterostructures(4). Lasing is measured from a transition-metal dichalcogenide heterobilayer (WSe2-MoSe2) integrated in a silicon nitride grating resonator. An abrupt increase in the spatial coherence of the emission is observed acrossthe lasing threshold. The work establishes interlayer excitons in two-dimensional heterostructures as a gain medium with spatially coherent lasing emission and potential for heterogeneous integration. With electrically tunable exciton-photon interaction strengths(5) and long-range dipolar interactions, these interlayer excitons are promising for application as low-power, ultrafast lasers and modulators and for the study of many-body quantum phenomena(6).
引用
收藏
页码:80 / +
页数:17
相关论文
共 34 条
[1]   CONDENSATION OF INDIRECT EXCITONS IN COUPLED ALAS/GAAS QUANTUM-WELLS [J].
BUTOV, LV ;
ZRENNER, A ;
ABSTREITER, G ;
BOHM, G ;
WEIMANN, G .
PHYSICAL REVIEW LETTERS, 1994, 73 (02) :304-307
[2]   Spatial Coherence and Stability in a Disordered Organic Polariton Condensate [J].
Daskalakis, K. S. ;
Maier, S. A. ;
Kena-Cohen, S. .
PHYSICAL REVIEW LETTERS, 2015, 115 (03)
[3]   Spatial coherence of a polariton condensate [J].
Deng, Hui ;
Solomon, Glenn S. ;
Hey, Rudolf ;
Ploog, Klaus H. ;
Yamamoto, Yoshihisa .
PHYSICAL REVIEW LETTERS, 2007, 99 (12)
[4]   Semiconductor nanowire lasers [J].
Eaton, Samuel W. ;
Fu, Anthony ;
Wong, Andrew B. ;
Ning, Cun-Zheng ;
Yang, Peidong .
NATURE REVIEWS MATERIALS, 2016, 1 (06)
[5]   Strong interlayer coupling in van der Waals heterostructures built from single-layer chalcogenides [J].
Fang, Hui ;
Battaglia, Corsin ;
Carraro, Carlo ;
Nemsak, Slavomir ;
Ozdol, Burak ;
Kang, Jeong Seuk ;
Bechtel, Hans A. ;
Desai, Sujay B. ;
Kronast, Florian ;
Unal, Ahmet A. ;
Conti, Giuseppina ;
Conlon, Catherine ;
Palsson, Gunnar K. ;
Martin, Michael C. ;
Minor, Andrew M. ;
Fadley, Charles S. ;
Yablonovitch, Eli ;
Maboudian, Roya ;
Javey, Ali .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2014, 111 (17) :6198-6202
[6]   High-temperature superfluidity with indirect excitons in van der Waals heterostructures [J].
Fogler, M. M. ;
Butov, L. V. ;
Novoselov, K. S. .
NATURE COMMUNICATIONS, 2014, 5
[7]   Van der Waals heterostructures [J].
Geim, A. K. ;
Grigorieva, I. V. .
NATURE, 2013, 499 (7459) :419-425
[8]   Millimeter-Scale Spatial Coherence from a Plasmon Laser [J].
Hoang, Thang B. ;
Akselrod, Gleb M. ;
Yang, Ankun ;
Odom, Teri W. ;
Mikkelsen, Maiken H. .
NANO LETTERS, 2017, 17 (11) :6690-6695
[9]   Observation of moire excitons in WSe2/WS2 heterostructure superlattices (vol 567, pg 76, 2019) [J].
Jin, Chenhao ;
Regan, Emma C. ;
Yan, Aiming ;
Utama, M. Iqbal Bakti ;
Wang, Danqing ;
Zhao, Sihan ;
Qin, Ying ;
Yang, Sijie ;
Zheng, Zhiren ;
Shi, Shenyang ;
Watanabe, Kenji ;
Taniguchi, Takashi ;
Tongay, Sefaattin ;
Zettl, Alex ;
Wang, Feng .
NATURE, 2019, 569 (7757) :E7-E7
[10]   Intrinsic transport properties of electrons and holes in monolayer transition-metal dichalcogenides [J].
Jin, Zhenghe ;
Li, Xiaodong ;
Mullen, Jeffrey T. ;
Kim, Ki Wook .
PHYSICAL REVIEW B, 2014, 90 (04)