Occurrence and congener profiles of polybrominated diphenyl ethers in green mussels (Perna viridis) collected from northern South China Sea and the associated potential health risk

被引:13
作者
Sun, Runxia [1 ]
Pan, Changgui [2 ,3 ]
Li, Qing X. [4 ]
Peng, Fengjiao [5 ]
Mai, Bixian [6 ]
机构
[1] Nanjing Univ Informat Sci & Technol, Sch Marine Sci, Nanjing 210044, Jiangsu, Peoples R China
[2] Guangxi Univ, Sch Marine Sci, Nanning 530004, Peoples R China
[3] Guangxi Univ, Guangxi Lab Study Coral Reefs South China Sea, Nanning 530004, Peoples R China
[4] Univ Hawaii Manoa, Dept Mol Biosci & Bioengn, 1955 East West Rd, Honolulu, HI 96822 USA
[5] Luxembourg Inst Hlth, Dept Populat Hlth, 1A B,Rue Thomas Edison, L-1445 Strassen, Luxembourg
[6] Chinese Acad Sci, State Key Lab Organ Geochem, Guangzhou Inst Geochemi, Guangzhou 510640, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
Polybroini nated diphenyl ethers; PBDE; Perna viridis; Pollution source; Congener profile; Health risk; PEARL RIVER ESTUARY; BROMINATED FLAME RETARDANTS; HALOGENATED ORGANIC POLLUTANTS; HUMAN DIETARY EXPOSURE; DECABROMODIPHENYL ETHER; SURFACE SEDIMENTS; GEOGRAPHICAL PATTERN; COASTAL WATERS; TEMPORAL TREND; ENNORE ESTUARY;
D O I
10.1016/j.scitotenv.2019.134276
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Polybrominated diphenyl ether (PBDE) contamination has become a major concern over the effects on human health. In the present study, we collected widely consumed green mussels (Perna viridis) samples from the northern South China Sea (NSCS) to investigate the occurrence, spatial distribution, congener profiles as well as potential risk of 18 PBDEs. All the target PBDEs were detected in green mussel samples, indicating their ubiquitous distribution. The concentrations of the total 18 PBDEs (Sigma PBDEs) in all samples varied from 6.96 to 55.6 ng/g lipid weight (lw), with BDE-47 and BDE-209 being the predominant PBDE congeners. Overall, the Sigma PBDEs pollution in green mussels from NSCS was at a moderate to high level in comparison with the PBDEs pollution worldwide. The dietary exposure of the local population in South China to PBDEs via consuming green mussels was estimated to be 0.30-0.80 ng/kg body weight (bw)/day. Evaluation of the exposure risk for BDE-47, 99, 153 and 209 indicated that health risks due to green mussel consumption are substantially lower than the US. EPA minimum concern level. (C) 2019 Elsevier B.V. All rights reserved.
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页数:8
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