Rapid simulations of hyperspectral near-field images of three-dimensional heterogeneous surfaces - part II

被引:21
作者
Chen, Xinzhong [1 ]
Yao, Ziheng [1 ]
Sun, Zhiyuan [2 ]
Stanciu, Stefan G. [3 ]
Basov, D. N. [4 ]
Hillenbrand, Rainer [5 ,6 ,7 ]
Liu, Mengkun [1 ,8 ]
机构
[1] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA
[2] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA
[3] Univ Politehn Bucuresti, Ctr Microscopy Microanal & Informat Proc, Bucharest 060042, Romania
[4] Columbia Univ, Dept Phys, New York, NY 10027 USA
[5] EHU UPV, CIC NanoGUNE BRTA, Donostia San Sebastian 20018, Spain
[6] EHU UPV, Dept Elect & Elect, Donostia San Sebastian 20018, Spain
[7] IKERBASQUE, Basque Fdn Sci, Bilbao 48011, Spain
[8] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA
基金
美国国家科学基金会;
关键词
EMISSION NANOSCOPY; ANALYTICAL-MODEL; LOSS POLARITONS; SPECTROSCOPY; MICROSCOPY; SCATTERING; CONTRAST; RECOVERY;
D O I
10.1364/OE.452949
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The modeling of the near-field interaction in the scattering-type scanning near-field optical microscope (s-SNOM) is rapidly advancing, although an accurate yet versatile modeling framework that can be easily adapted to various complex situations is still lacking. In this work, we propose a time-efficient numerical scheme in the quasi-electrostatic limit to capture the tip-sample interaction in the near field. This method considers an extended tip geometry, which is a significant advantage compared to the previously reported method based on the point-dipole approximation. Using this formalism, we investigate, among others, nontrivial questions such as uniaxial and biaxial anisotropy in the near-field interaction, the relationship between various experimental parameters (e.g. tip radius, tapping amplitude, etc.), and the tip-dependent spatial resolution. The demonstrated method further sheds light on the understanding of the contrast mechanism in s-SNOM imaging and spectroscopy, while also representing a valuable platform for future quantitative analysis of the experimental observations. (C) 2022 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
引用
收藏
页码:11228 / 11242
页数:15
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