Gas diffusion electrodes (GDEs) for electrochemical reduction of carbon dioxide, carbon monoxide, and dinitrogen to value-added products: a review
被引:345
作者:
Rabiee, Hesamoddin
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Univ Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, AustraliaUniv Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, Australia
Rabiee, Hesamoddin
[1
]
Ge, Lei
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Univ Southern Queensland, Ctr Future Mat, Springfield Cent, Qld 4300, Australia
Univ Queensland, Sch Chem Engn, Brisbane, Qld 4072, AustraliaUniv Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, Australia
Ge, Lei
[2
,3
]
Zhang, Xueqin
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Univ Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, AustraliaUniv Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, Australia
Zhang, Xueqin
[1
]
Hu, Shihu
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Univ Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, AustraliaUniv Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, Australia
Hu, Shihu
[1
]
Li, Mengran
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Univ Queensland, Sch Chem Engn, Brisbane, Qld 4072, AustraliaUniv Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, Australia
Li, Mengran
[3
]
Yuan, Zhiguo
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Univ Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, AustraliaUniv Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, Australia
Yuan, Zhiguo
[1
]
机构:
[1] Univ Queensland, Fac Engn Architecture & Informat Technol, Adv Water Management Ctr, St Lucia, Qld 4072, Australia
[2] Univ Southern Queensland, Ctr Future Mat, Springfield Cent, Qld 4300, Australia
[3] Univ Queensland, Sch Chem Engn, Brisbane, Qld 4072, Australia
MEMBRANE FUEL-CELLS;
ELECTROCATALYTIC CO2 REDUCTION;
GENERAL TECHNOECONOMIC ANALYSIS;
HABER-BOSCH PROCESS;
POLYMER ELECTROLYTE;
OXYGEN REDUCTION;
NITROGEN REDUCTION;
LARGE-SCALE;
EFFICIENT CO2;
FORMIC-ACID;
D O I:
10.1039/d0ee03756g
中图分类号:
O6 [化学];
学科分类号:
0703 ;
摘要:
Electrochemical reduction of gaseous feeds such as CO2, CO, and N-2 holds promise for sustainable energy and chemical production. Practical application of this technology is impeded by slow mass transport of the sparingly soluble gases to conventional planar electrodes. Gas diffusion electrodes (GDEs) maintain a high gas concentration in the vicinity of the catalyst and improve mass transport, thereby resulting in current densities higher by orders of magnitude. However, gaseous feeds cause changes to the GDE environment, and specific features are required to efficiently tune the product selectivity and improve reaction stability. Herein, with a comprehensive review of the challenges and advances in GDE development for various electrocatalytic reactions, we intend to complement the body of material-focused reviews. This review outlines GDE fundamentals and highlights key advantages of GDE over conventional electrodes. Through critical discussion about steps in GDE fabrication, and specific shortcomings and remedial strategies for various electrochemical applications, this review discusses connections, unique design criteria, and potential opportunities for gas-fed reactions and desired products. Finally, priorities for future studies are suggested, to support the advancement and scale-up of GDE-based electrochemical technologies.
机构:
IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Alcaide, Francisco
Alvarez, Garbine
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IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Alvarez, Garbine
Cabot, Pere L.
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Univ Barcelona, Fac Chem, Dept Mat Sci & Phys Chem, Lab Mat & Environm Elect,Sect Phys Chem, Marti & Franques 1-11, Barcelona 08028, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Cabot, Pere L.
Genova-Koleva, Radostina
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Univ Barcelona, Fac Chem, Dept Mat Sci & Phys Chem, Lab Mat & Environm Elect,Sect Phys Chem, Marti & Franques 1-11, Barcelona 08028, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Genova-Koleva, Radostina
Grande, Hans-Juergen
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IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Grande, Hans-Juergen
Miguel, Oscar
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机构:
IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
机构:
IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Alcaide, Francisco
Alvarez, Garbine
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h-index: 0
机构:
IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Alvarez, Garbine
Cabot, Pere L.
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h-index: 0
机构:
Univ Barcelona, Fac Chem, Dept Mat Sci & Phys Chem, Lab Mat & Environm Elect,Sect Phys Chem, Marti & Franques 1-11, Barcelona 08028, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Cabot, Pere L.
Genova-Koleva, Radostina
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机构:
Univ Barcelona, Fac Chem, Dept Mat Sci & Phys Chem, Lab Mat & Environm Elect,Sect Phys Chem, Marti & Franques 1-11, Barcelona 08028, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Genova-Koleva, Radostina
Grande, Hans-Juergen
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h-index: 0
机构:
IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain
Grande, Hans-Juergen
Miguel, Oscar
论文数: 0引用数: 0
h-index: 0
机构:
IK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, SpainIK4 CIDETEC, Div Energy, P Miramon196, San Sebastian 20009, Spain