Evolutionary optimization of three-photon absorption in molecular iodine

被引：1
|
作者：
Burbidge, Robert [1 ]
Rowland, Jem J. [1 ]
King, Ross D. [1 ]
Form, Nicholas T. [2 ]
Whitaker, Benjamin J. [2 ]
机构：
[1] Univ Wales, Dept Comp Sci, Aberystwyth SY23 3DB, Dyfed, Wales
[2] Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England
来源：
2007 IEEE SYMPOSIUM ON COMPUTATIONAL INTELLIGENCE AND DATA MINING, VOLS 1 AND 2 | 2007年
基金：
英国工程与自然科学研究理事会;
关键词：
D O I：
10.1109/CIDM.2007.368858
中图分类号：
TP18 [人工智能理论];
学科分类号：
081104 ; 0812 ; 0835 ; 1405 ;
摘要：
We report on the application or an evolutionary algorithm to a noisy, dynamic optimization problem in chemistry: the maximization of three-photon absorption in molecular iodine. An evolution strategy is used in real-time in a closed loop experiment to search the space of physically realizable phase-modulated femtosecond laser pulses. The probability of three-photon absorption is estimated by measuring UV fluorescence. With the evolutionary search it is possible to enhance the UV fluorescence by a factor of 3.4 compared to the most intense pulse.
引用
收藏
页码：96 / 100
页数：5
相关论文
共 50 条
  • [1] Enhancing the probability of three-photon absorption in iodine through pulse shaping
    Form, N. T.
    Whitaker, B. J.
    Meier, C.
    JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2008, 41 (07)
  • [2] Three-photon absorption in InAs
    Hasselbeck, MP
    Said, AA
    van Stryland, EW
    Sheik-Bahae, M
    OPTICAL AND QUANTUM ELECTRONICS, 1998, 30 (03) : 193 - 200
  • [3] Three-Photon Absorption in InAs
    M. P. Hasselbeck
    A. A. Said
    E. W. van Stryland
    M. Sheik-Bahae
    Optical and Quantum Electronics, 1998, 30 : 193 - 200
  • [4] Three-photon absorption materials and applications
    Lu, Changgui
    Cui, Yiping
    NONLINEAR OPTICS: TECHNOLOGIES AND APPLICATIONS, 2008, 6839 : U521 - U528
  • [5] Two-photon and three-photon absorption in dinaphthoporphycenes
    Rao, S. Venugopal
    Prashant, T. Shuvan
    Swain, Debasis
    Sarma, Tridib
    Panda, Pradeepta K.
    Tewari, Surya P.
    CHEMICAL PHYSICS LETTERS, 2011, 514 (1-3) : 98 - 103
  • [6] Three-photon absorption cross-section of simple molecular liquids
    Naskrecki, R
    Menard, M
    van der Meulen, P
    Vigneron, G
    Pommeret, S
    OPTICS COMMUNICATIONS, 1998, 153 (1-3) : 32 - 38
  • [7] Three-photon absorption in ZnO and ZnS crystals
    He, J
    Qu, YL
    Li, HP
    Mi, J
    Ji, W
    OPTICS EXPRESS, 2005, 13 (23): : 9235 - 9247
  • [8] Observation of three-photon enhanced four-photon absorption
    Yoshino, F
    Polyakov, S
    Liu, MG
    Stegeman, G
    PHYSICAL REVIEW LETTERS, 2003, 91 (06)
  • [9] Two-photon and three-photon absorption in an organometallic dendrimer
    Samoc, Marek
    Morrall, Joseph P.
    Dalton, Gulliver T.
    Cifuentes, Marie P.
    Humphrey, Mark G.
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2007, 46 (05) : 731 - 733
  • [10] Ab initio calculations of three-photon absorption
    Cronstrand, P
    Luo, Y
    Norman, P
    Ågren, H
    CHEMICAL PHYSICS LETTERS, 2003, 375 (1-2) : 233 - 239
12345