Binary TiO2/reduced graphene oxide nanocomposite for improving methylene blue photodegradation

被引:12
作者
Dinh Ngoc Trinh [1 ,2 ,3 ]
Thieu Quang Quoc Viet [1 ,2 ,3 ,5 ]
Tran Huynh Nhu [1 ,2 ,3 ]
Nguyen Minh Dat [1 ,3 ]
Doan Ba Thinh [2 ,3 ]
Nguyen Duy Hai [2 ,3 ]
Le Tan Tai [2 ,3 ]
Doan Thi Yen Oanh [4 ]
Vu Hoang Khoi [2 ,3 ]
Hoang Minh Nam [2 ,3 ]
Mai Thanh Phong [2 ,3 ]
Nguyen Huu Hieu [1 ,2 ,3 ]
机构
[1] Ho Chi Minh City Univ Technol, VNU HCM Key Lab Chem Engn & Petr Proc, Key CEPP Lab, 268 Ly Thuong Kiet St,Dist 10, Ho Chi Minh City 70000, Vietnam
[2] Ho Chi Minh City Univ Technol, Fac Chem Engn, 268 Ly Thuong Kiet St, Ho Chi Minh City 70000, Vietnam
[3] Vietnam Natl Univ Ho Chi Minh City, Ho Chi Minh City 70000, Vietnam
[4] Vietnam Acad Sci & Technol, Publishing House Sci Technol, 18 Hoang Quoc Viet, Hanoi 10000, Vietnam
[5] Can Tho Univ, Coll Engn Technol, 3-2 Str, Can Tho City 90000, Vietnam
关键词
TiO2; rGO; hydrothermal; methylene blue; adsorption; photodegradation; PHOTOCATALYTIC DEGRADATION; TIO2-RGO COMPOSITE; PERFORMANCE; GRAPHITE; PHENOL; WATER;
D O I
10.1002/vjch.202100009
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Herein, TiO2/reduced graphene oxide (TiO2/rGO) nanocomposites were fabricated using the hydrothermal method and investigated with the amount of titanium precursors. The binary nanocomposites were characterized by modern analysis method. The adsorption capacity and photocatalyst degradation were performed based on methylene blue. The appropriate as-prepared material with 1.5 mL TIP contained a large specific surface area (110.549 m(2)/g) with TiO2 ranging 4-25 nm homogenously grafting on the rGO surface. The adsorption results were shown in good accordance with the pseudo-second-order while the photoreaction kinetics pursued the pseudo-first-order with a high-rate constant. After the adsorption state, the yield reaches 62.1 % and under UV light for 90 min, 96.8 % of MB was efficiently degraded from water media, which showed a more impressive effect as compared with P25 and rGO. Therefore, the use of TiO2/rGO could be applied in the mass-scale treatment of organic pollutants in wastewater.
引用
收藏
页码:395 / 404
页数:10
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