3D reconstruction of a gas diffusion layer and a microporous layer

被引:152
作者
Ostadi, H. [1 ]
Rama, P. [2 ]
Liu, Y. [2 ]
Chen, R. [2 ]
Zhang, X. X. [3 ]
Jiang, K. [1 ]
机构
[1] Univ Birmingham, Ctr Biomed & Nanotechnol, Sch Mech & Mfg Engn, Birmingham B15 2TT, W Midlands, England
[2] Univ Loughborough, Dept Aeronaut & Automot Engn, Loughborough LE11 3TU, Leics, England
[3] Univ Liverpool, Dept Engn, Liverpool L69 3GH, Merseyside, England
关键词
Gas diffusion layer; Microporous layer; FIB/SEM nano-tomography; X-ray nano-tomography; Lattice Boltzmann numerical modeling; MATHEMATICAL-MODEL; WATER-SATURATION; TRANSPORT; PERMEABILITY;
D O I
10.1016/j.memsci.2010.01.031
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The focus of the current study is on a state-of-the-art twin-layer gas diffusion layer (GDL) which consists of carbon tissues with a fibre diameter of 5-20 mu m, and contains a microporous layer (MPL) coating which has sub-micron porous features. In the current study, real-world digital three-dimensional images of the GDL-MPL assembly are created through X-ray nano-tomography with a 680 nm pixel resolution for the GDL and focused ion beam/scanning electron microscopy (FIB/SEM) nano-tomography with a 14 nm pixel resolution for the MPL The critical nano-structural features including porosity, characteristic lengths and 3D pore size distribution are determined directly from the 3D digital representation. In addition to morphological parameters, the FIB/SEM nano-tomography technique has been combined with lattice Boltzmann (LB) numerical modelling in order to calculate the tortuosity and permeability of the MPL (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:69 / 74
页数:6
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