Effect of pH on absorption spectra of photogenerated holes in nanocrystalline TiO2 films

被引:50
作者
Yoshihara, Toshitada [1 ]
Tamaki, Yoshiaki [1 ]
Furube, Akihiro [1 ]
Murai, Miki [1 ]
Hara, Kohjiro [1 ]
Katoh, Ryuzi [1 ]
机构
[1] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058565, Japan
关键词
D O I
10.1016/j.cplett.2007.03.017
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We have measured transient absorption spectra of TiO2 under several pH conditions. We successfully extracted the spectral contribution of two different trapped holes from the transient absorption spectra. Based on the results, we discuss the origin of absorption spectra of holes in TiO2. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:268 / 273
页数:6
相关论文
共 28 条
[1]   ABSORPTION SPECTRA OF DIMER CATIONS .1. OLEFINS [J].
BADGER, B ;
BROCKLEH.B .
TRANSACTIONS OF THE FARADAY SOCIETY, 1969, 65 (562P) :2576-&
[2]   FLASH-PHOTOLYSIS OBSERVATION OF THE ABSORPTION-SPECTRA OF TRAPPED POSITIVE HOLES AND ELECTRONS IN COLLOIDAL TIO2 [J].
BAHNEMANN, D ;
HENGLEIN, A ;
LILIE, J ;
SPANHEL, L .
JOURNAL OF PHYSICAL CHEMISTRY, 1984, 88 (04) :709-711
[3]   Charge carrier dynamics at TiO2 particles: Reactivity of free and trapped holes [J].
Bahnemann, DW ;
Hilgendorff, M ;
Memming, R .
JOURNAL OF PHYSICAL CHEMISTRY B, 1997, 101 (21) :4265-4275
[4]  
Barbe CJ, 1997, J AM CERAM SOC, V80, P3157, DOI 10.1111/j.1151-2916.1997.tb03245.x
[5]   THEORETICAL-ANALYSIS OF THE STRUCTURES OF TITANIUM-DIOXIDE CRYSTALS [J].
FAHMI, A ;
MINOT, C ;
SILVI, B ;
CAUSA, M .
PHYSICAL REVIEW B, 1993, 47 (18) :11717-11724
[6]  
Fujishima A., 2000, Journal of Photochemistry and Photobiology C: Photochemistry Reviews, V1, P1, DOI [10.1016/S1389-5567(00)00002-2, DOI 10.1016/S1389-5567(00)00002-2]
[7]  
FURUBE A, 1997, CHEM HYS LETT, V275, P234
[8]   Highly efficient photon-to-electron conversion with mercurochrome-sensitized nanoporous oxide semiconductor solar cells [J].
Hara, K ;
Horiguchi, T ;
Kinoshita, T ;
Sayama, K ;
Sugihara, H ;
Arakawa, H .
SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2000, 64 (02) :115-134
[9]   ENVIRONMENTAL APPLICATIONS OF SEMICONDUCTOR PHOTOCATALYSIS [J].
HOFFMANN, MR ;
MARTIN, ST ;
CHOI, WY ;
BAHNEMANN, DW .
CHEMICAL REVIEWS, 1995, 95 (01) :69-96
[10]   ABSORPTION-SPECTRA OF DIMER CATIONS AND OTHER CATIONIC SPECIES PRODUCED BY WARMING OF GAMMA-IRRADIATED GLASSY SOLUTIONS OF AROMATIC-HYDROCARBONS [J].
KIRA, A ;
IMAMURA, M .
JOURNAL OF PHYSICAL CHEMISTRY, 1979, 83 (17) :2267-2273