Fast sound in expanded fluid Hg accompanying the metal-nonmetal transition

被引:43
作者
Ishikawa, D [1 ]
Inui, M
Matsuda, K
Tamura, K
Tsutsui, S
Baron, AQR
机构
[1] Kyoto Univ, Grad Sch Engn, Kyoto 6068501, Japan
[2] RIKEN, SPring 8, Mikazuki, Hyogo 6795148, Japan
[3] Hiroshima Univ, Fac Integrated Arts & Sci, Higashihiroshima 7398521, Japan
[4] JASRI, SPring 8, Mikazuki, Hyogo 6795198, Japan
关键词
D O I
10.1103/PhysRevLett.93.097801
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The dynamic structure factor S(Q,omega) of expanded fluid Hg has been measured up to the metal-nonmetal transition region at 9.0 g cm(-3) (1723 K and 1940 bars) using high-resolution inelastic x-ray scattering, at momentum transfers, Q, from 0.2 to 4.8 Angstrom(-1). Analysis in the framework of generalized hydrodynamics reveals that the frequencies of the collective excitations increase faster with Q than estimated from the macroscopic speed of sound. The effective sound velocity at 9.0 g cm(-3) estimated from the dispersion relation is triple the ultrasonic sound velocity. The present result suggests the existence of fast sound in expanded fluid Hg accompanying the metal-nonmetal transition.
引用
收藏
页码:097801 / 1
页数:4
相关论文
共 25 条
[1]   FAST SOUND IN LIQUID WATER [J].
BALUCANI, U ;
RUOCCO, G ;
TORCINI, A ;
VALLAURI, R .
PHYSICAL REVIEW E, 1993, 47 (03) :1677-1684
[2]   Early commissioning of the SPring-8 beamline for high resolution inelastic X-ray scattering [J].
Baron, AQR ;
Tanaka, Y ;
Miwa, D ;
Ishikawa, D ;
Mochizuki, T ;
Takeshita, K ;
Goto, S ;
Matsushita, T ;
Kimura, H ;
Yamamoto, F ;
Ishikawa, T .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2001, 467 :627-630
[3]  
Boon J. P., 1980, MOL HYDRODYNAMICS
[4]   OBSERVATION OF COLLECTIVE EXCITATIONS IN HEAVY-WATER IN 108 CM-1 MOMENTUM RANGE [J].
BOSI, P ;
DUPRE, F ;
MENZINGER, F ;
SACCHETTI, F ;
SPINELLI, MC .
LETTERE AL NUOVO CIMENTO, 1978, 21 (12) :436-440
[5]   Neutron investigation of the ion dynamics in liquid mercury: Evidence for collective excitations [J].
Bove, LE ;
Sacchetti, F ;
Petrillo, C ;
Dorner, B ;
Formisano, F ;
Barocchi, F .
PHYSICAL REVIEW LETTERS, 2001, 87 (21) :215504-1
[6]  
FAK B, 1992, 92FA008S I LOUE LANG
[7]  
GOZLAFF W, 1988, Z PHYS CHEM, V156, P219
[8]  
HENSEL F, 1999, FLUID METALS
[9]   Collective dynamics of liquid Hg investigated by inelastic X-ray scattering [J].
Hosokawa, S ;
Sinn, H ;
Hensel, F ;
Alatas, A ;
Alp, EE ;
Pilgrim, WC .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 2002, 312-14 :163-167
[10]   Local structure of expanded fluid mercury using synchrotron radiation: From liquid to dense vapor [J].
Inui, M ;
Hong, XG ;
Tamura, K .
PHYSICAL REVIEW B, 2003, 68 (09)