Terahertz Photoconductivity Spectra of Electrodeposited Thin Bi Films

被引:3
作者
Nevinskas, Ignas [1 ]
Mockus, Zenius [1 ]
Juskenas, Remigijus [1 ]
Norkus, Ricardas [1 ]
Selskis, Algirdas [1 ]
Norkus, Eugenijus [1 ]
Krotkus, Atunas [1 ]
机构
[1] Ctr Phys Sci & Technol, Sauletekio Al 3, LT-10257 Vilnius, Lithuania
关键词
bismuth film; electrodeposition; terahertz emission; terahertz photoconductivity spectra; femtosecond laser; CO2; REDUCTION; BISMUTH; NANOSHEETS; CU;
D O I
10.3390/ma14123150
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Electron dynamics in the polycrystalline bismuth films were investigated by measuring emitted terahertz (THz) radiation pulses after their photoexcitation by tunable wavelength femtosecond duration optical pulses. Bi films were grown on metallic Au, Pt, and Ag substrates by the electrodeposition method with the Triton X-100 electrolyte additive, which allowed us to obtain more uniform films with consistent grain sizes on any substrate. It was shown that THz pulses are generated due to the spatial separation of photoexcited electrons and holes diffusing from the illuminated surface at different rates. The THz photoconductivity spectra analysis has led to a conclusion that the thermalization of more mobile carriers (electrons) is dominated by the carrier-carrier scattering rather than by their interaction with the lattice.
引用
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页数:9
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