Influence of temperature on corrosion behavior, wettability, and surface conductivity of 304 stainless steel in simulated cathode environment of proton exchange membrane fuel cells

被引：28

作者：

Xuan, Junji ^{[1
,2
]}

Xu, Likun ^{[1
,2
]}

Bai, Shuangfeng ^{[2
]}

Zhao, Ting ^{[2
]}

Xin, Yonglei ^{[2
]}

Zhang, Guodong ^{[3
]}

Xue, Lili ^{[1
]}

Li, Li ^{[1
]}

机构：

[1] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Peoples R China

[2] Luoyang Ship Mat Res Inst, State Key Lab Marine Corros & Protect, Qingdao 266237, Peoples R China

[3] Wuhan Univ, Sch Power & Mech Engn, Wuhan 430072, Peoples R China

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2021年 / 46卷 / 44期

关键词：

Bipolar plate; Corrosion; Proton exchange membrane fuel cell; (PEMFC); Stainless steel; Wettability; Interfacial contact resistance (ICR); BIPOLAR PLATE MATERIAL; 316L STAINLESS-STEEL; PASSIVE FILMS; AISI; 304-STAINLESS-STEEL; COATINGS; RESISTANCE; SS316L; PERFORMANCE; PROTECTION; ELECTRODEPOSITION;

D O I：

10.1016/j.ijhydene.2021.04.119

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The effects of temperature on corrosion behavior, wettability, and surface conductivity of 304 stainless steel (SS304) in simulated cathode environment of proton exchange membrane fuel cells (PEMFC) are investigated systematically using electrochemical tests and surface analyses. The results indicate that although the corrosion resistance of SS304 is decreased with the rising of solution temperature, the current density of SS304 at the working potential in the simulated PEMFC cathode environment can still meet the 2025 U.S. Department of Energy (DOE) technical target (i(corr) < 1 mu A cm(-2)). Meanwhile, the surface wettability and ICR of SS304 samples after potentiostatic polarization show a continuous increase with the rise of the simulated solution temperature. The surface conductivity of SS304 both before and after polarization cannot reach the 2025 DOE technical target (<0.01 Omega cm(2)) and needs to be improved by surface modification. (C) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

引用

页码：22920 / 22931

页数：12

共 68 条

[1] Effect of Plastic Deformation on Passivation Characteristics of Type 304 Stainless Steel [J].

Ahmedabadi, Parag M. ;

Kain, Vivekanand ;

Agrawal, Ashika .

JOURNAL OF MATERIALS ENGINEERING AND PERFORMANCE, 2019, 28 (11) :7036-7046

[2] Time dependency of the hydrophilicity and hydrophobicity of metallic alloys subjected to femtosecond laser irradiations [J].

Bizi-bandoki, P. ;

Valette, S. ;

Audouard, E. ;

Benayoun, S. .

APPLIED SURFACE SCIENCE, 2013, 273 :399-407

[3] EIS evaluation of steady-state characteristic of 316L stainless steel passive film grown in acidic solution [J].

Boissy, C. ;

Alemany-Dumont, C. ;

Normand, B. .

ELECTROCHEMISTRY COMMUNICATIONS, 2013, 26 :10-12

[4] Development and performance evaluation of a high temperature proton exchange membrane fuel cell with stamped 304 stainless steel bipolar plates [J].

Chen, Chen-Yu ;

Su, Sheng-Chun .

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2018, 43 (29) :13430-13439

[5] Electrochemical Properties of Niobium Modified AISI316L Stainless Steel Bipolar Plates for Direct Formic Acid Fuel Cell [J].

Cui, Y. F. ;

Cui, J. L. ;

Xu, X. ;

Cheng, F. P. ;

Wang, L. X. ;

Li, S. ;

Ji, S. J. ;

Sun, J. C. .

FUEL CELLS, 2017, 17 (05) :698-707

[6] Review of materials and processing methods used in the production of bipolar plates for fuel cells [J].

Cunningham, B. D. ;

Huang, J. ;

Baird, D. G. .

INTERNATIONAL MATERIALS REVIEWS, 2007, 52 (01) :1-13

[7] Surface and corrosion properties of modified passive layer on 304 stainless steel as bipolar plates for PEMFCs [J].

Dadfar, M. ;

Salehi, M. ;

Golozar, M. A. ;

Trasatti, S. ;

Casaletto, M. P. .

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (41) :25869-25876

[8] Surface modification of 304 stainless steels to improve corrosion behavior and interfacial contact resistance of bipolar plates [J].

Dadfar, M. ;

Salehi, M. ;

Golozar, M. A. ;

Trasatti, S. .

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2016, 41 (46) :21375-21384

[9] Review of the membrane and bipolar plates materials for conventional and unitized regenerative fuel cells [J].

Dihrab, Salwan S. ;

Sopian, K. ;

Alghoul, M. A. ;

Sulaiman, M. Y. .

RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2009, 13 (6-7) :1663-1668

[10] Carbon coated stainless steel bipolar plates in polymer electrolyte membrane fuel cells [J].

Feng, Kai ;

Cai, Xun ;

Sun, Hailin ;

Li, Zhuguo ;

Chu, Paul K. .

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