Visible light activated photocatalytic degradation of tetracycline by a magnetically separable composite photocatalyst: Graphene oxide/magnetite/cerium-doped titania

被引:192
作者
Cao, Muhan [1 ]
Wang, Peifang [1 ]
Ao, Yanhui [1 ]
Wang, Chao [1 ]
Hou, Jun [1 ]
Qian, Jin [1 ]
机构
[1] Hohai Univ, Coll Environm, Minist Educ, Key Lab Integrated Regulat & Resource Dev Shallow, Nanjing 210098, Jiangsu, Peoples R China
基金
美国国家科学基金会; 中国国家自然科学基金;
关键词
Ce-doped TiO2; Magnetically separable; Graphene oxide; Tetracyclines; Photocatalysis; CARBON NANOTUBES; AQUEOUS-SOLUTION; ANTIBIOTIC TETRACYCLINE; HYBRID PHOTOCATALYSTS; ADSORPTION; PERFORMANCE; TOXICITY; REMOVAL; MECHANISMS; PRODUCTS;
D O I
10.1016/j.jcis.2016.01.005
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this study, magnetic graphene oxide-loaded Ce-doped titania (MGO-Ce-TiO2) hybridized composite was prepared by a facile method. The as-prepared samples exhibited good adsorption capacity, high visible-light photoactive and magnetic separability as a novel photocatalyst in the degradation of tetracyclines (TC). The intermediate products and photocatalytic route of TC were proposed based on the analysis results of LC-MS. Moreover, the repeatability of the photoactivity with the use of MGO-Ce-TiO2 was investigated in the multi-round experiments with the assistance of an applied magnetic field. Therefore, the prepared composite photocatalysts were considered as a kind of promising photocatalyst in a suspension reaction system, in which they can offer effectively recovery ability. The effect of MGO content on the photocatalytic performance was also studied, and an optimum content was obtained. (C) 2016 Elsevier Inc. All rights reserved.
引用
收藏
页码:129 / 139
页数:11
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