Why does 2-(2-aminoethylamino)ethanol have superior CO2 separation performance to monoethanolamine? A computational study

被引:8
作者
Aso, Daiki [1 ]
Orimoto, Yuuichi [2 ]
Higashino, Makoto [3 ]
Taniguchi, Ikuo [4 ]
Aoki, Yuriko [2 ]
机构
[1] Kyushu Univ, Interdisciplinary Grad Sch Engn Sci, Dept Mol & Mat Sci, 6-1 Kasuga Pk, Fukuoka 8168580, Japan
[2] Kyushu Univ, Fac Engn Sci, Dept Adv Mat Sci & Engn, 6-1 Kasuga Pk, Fukuoka 8168580, Japan
[3] Oita Coll, Natl Inst Technol, Dept Civil & Environm Engn, 1666 Maki, Oita 8700152, Japan
[4] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan
关键词
CARBON-DIOXIDE; CAPTURE; ABSORPTION; PHASE; AEEA;
D O I
10.1039/d2cp01136k
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Our computational reaction analysis shows that 2-(2-aminoethylamino)ethanol (AEEA) has superior performance to monoethanolamine for CO2 separation, in terms of its ability to sorb CO2 by its primary amine and desorb CO2 by its secondary amine.
引用
收藏
页码:14172 / 14176
页数:5
相关论文
共 29 条
[1]   Computational approach for investigating the mechanism of carbon dioxide interaction by 2-(2-aminoethylamino)ethanol: A significant role of water molecule [J].
Aso, Daiki ;
Orimoto, Yuuichi ;
Higashino, Makoto ;
Taniguchi, Ikuo ;
Aoki, Yuriko .
CHEMICAL PHYSICS LETTERS, 2021, 783
[2]   Carbon capture and storage update [J].
Boot-Handford, M. E. ;
Abanades, J. C. ;
Anthony, E. J. ;
Blunt, M. J. ;
Brandani, S. ;
Mac Dowell, N. ;
Fernandez, J. R. ;
Ferrari, M. -C. ;
Gross, R. ;
Hallett, J. P. ;
Haszeldine, R. S. ;
Heptonstall, P. ;
Lyngfelt, A. ;
Makuch, Z. ;
Mangano, E. ;
Porter, R. T. J. ;
Pourkashanian, M. ;
Rochelle, G. T. ;
Shah, N. ;
Yao, J. G. ;
Fennell, P. S. .
ENERGY & ENVIRONMENTAL SCIENCE, 2014, 7 (01) :130-189
[3]  
Dennington I. I., 2000, GaussView
[4]  
Frisch M. J., 2013, GAUSSIAN09 REVISION
[5]   THE PATH OF CHEMICAL-REACTIONS - THE IRC APPROACH [J].
FUKUI, K .
ACCOUNTS OF CHEMICAL RESEARCH, 1981, 14 (12) :363-368
[6]   Proton Transfer from the Inactive Gas-Phase Nicotine Structure to the Bioactive Aqueous-Phase Structure [J].
Gaigeot, Marie-Pierre ;
Cimas, Alvaro ;
Seydou, Mahamadou ;
Kim, Ju-Young ;
Lee, Sungyul ;
Schermann, Jean-Pierre .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (51) :18067-18077
[7]   Carbon capture and storage [J].
Gibbins, Jon ;
Chalmers, Hannah .
ENERGY POLICY, 2008, 36 (12) :4317-4322
[8]   A 13C NMR study of carbon dioxide absorption and desorption in pure and blended 2-(2-aminoethylamine)ethanol (AEEA) and 2-amino-2-methyl-1-propanol (AMP) solutions [J].
Guo, Chao ;
Chen, Shaoyun ;
Zhang, Yongchun .
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2014, 28 :88-95
[9]   Acceleration of rises in the level of rivers induced by rising air temperatures in a cold climate [J].
Higashino, Makoto ;
Aso, Daiki ;
Stefan, Heinz G. .
SCIENCE OF THE TOTAL ENVIRONMENT, 2021, 794
[10]   Reaction mechanisms of aqueous monoethanolamine with carbon dioxide: a combined quantum chemical and molecular dynamics study [J].
Hwang, Gyeong S. ;
Stowe, Haley M. ;
Paek, Eunsu ;
Manogaran, Dhivya .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2015, 17 (02) :831-839