The impact of wood smoke on ambient PM2.5 in northern Rocky Mountain valley communities

被引:50
作者
Ward, Tony [1 ]
Lange, Todd [2 ]
机构
[1] Univ Montana, Ctr Environm Hlth Sci, Missoula, MT 59812 USA
[2] Univ Arizona, NSF, Arizona AMS Facil, Tucson, AZ USA
关键词
Chemical mass balance; Woodstoves; Source apportionment; Biomass smoke; PM2.5; CHEMICAL MASS-BALANCE; SECONDARY ORGANIC AEROSOL; SOURCE APPORTIONMENT; RECEPTOR MODELS; AIR-POLLUTION; EMISSIONS; CALIFORNIA; SENSITIVITY; WASHINGTON; MISSOULA;
D O I
10.1016/j.envpol.2009.10.016
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
During the winters of 2006/2007 and 2007/2008, PM2.5 source apportionment programs were carried out within five western Montana valley communities Filter samples were analyzed for mass and chemical composition information was utilized in a Chemical Mass Balance (CMB) computer model to apportion the sources of PM2.5 Results showed that wood smoke (likely residential woodstoves) was the major source of PM2.5 in each of the communities, contributing from 56% to 77% of the measured wintertime PM2.5 Results of C-14 analyses showed that between 44% and 76% of the measured PM2.5 came from a new carbon (wood smoke) source, confirming the results of the CMB modeling In summary, the CMB model results, coupled with the C-14 results, support that wood smoke is the major contributor to the overall PM2.5 mass in these rural, northern Rocky Mountain airsheds throughout the winter months (C) 2009 Elsevier Ltd All rights reserved
引用
收藏
页码:723 / 729
页数:7
相关论文
共 35 条
[1]  
[Anonymous], 2020, Gothenburg Protocol to reduce transboundary air pollution, DOI DOI 10.5860/CHOICE.44-4512
[2]  
Carlson J, 1990, PM10 CHEM MASS BALAN
[3]   Wood burning impact on PM10 in three Austrian regions [J].
Caseiro, Alexandre ;
Bauer, Heidi ;
Schmidl, Christoph ;
Pio, Casimiro A. ;
Puxbaum, Hans .
ATMOSPHERIC ENVIRONMENT, 2009, 43 (13) :2186-2195
[4]   Evaluation of organic markers for chemical mass balance source apportionment at the Fresno Supersite [J].
Chow, J. C. ;
Watson, J. G. ;
Lowenthal, D. H. ;
Chen, L. W. A. ;
Zielinska, B. ;
Mazzoleni, L. R. ;
Magliano, K. L. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (07) :1741-1754
[5]   RECEPTOR ORIENTED METHODS OF AIR PARTICULATE SOURCE APPORTIONMENT [J].
COOPER, JA ;
WATSON, JG .
JOURNAL OF THE AIR POLLUTION CONTROL ASSOCIATION, 1980, 30 (10) :1116-1125
[6]   A fuel-based inventory for heavy-duty diesel truck emissions [J].
Dreher, DB ;
Harley, RA .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 1998, 48 (04) :352-358
[8]   Detection of excess ammonia emissions from in-use vehicles and the implications for fine particle control [J].
Fraser, MP ;
Cass, GR .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (08) :1053-1057
[9]   CHEMICAL ELEMENT BALANCES AND IDENTIFICATION OF AIR-POLLUTION SOURCES [J].
FRIEDLANDER, SK .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1973, 7 (03) :235-240
[10]  
GELENCSER A, 2007, J GEOPHYS RES-ATMOS, V112