Discharge characteristics of plasma induced by water drop and its potential for water treatment

被引:23
作者
Wang, Xiaoping [1 ]
Zhao, Dengmei [1 ]
Tan, Xuemei [1 ]
Chen, Yixia [1 ]
Chen, Zihan [1 ]
Xiao, He [1 ]
机构
[1] Chongqing Technol & Business Univ, Coll Environm & Resources, Chongqing Key Lab Catalysis & Environm New Mat, Chongqing 400067, Peoples R China
基金
中国国家自然科学基金;
关键词
Water drop induced discharge; Plasma; Water treatment; Ibuprofen removal; DIELECTRIC BARRIER DISCHARGE; CORONA-STREAMER DISCHARGE; FLUE-GAS DESULFURIZATION; SURFACE DISCHARGE; SULFITE OXIDATION; PULSED DISCHARGE; DEGRADATION; AIR; REACTORS; SPRAY;
D O I
10.1016/j.cej.2017.07.082
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Water surface discharge is an effective water treatment method. However, the industrial application of this technology is limited by some problems including the difficulty to get a large area of uniform discharge plasma and the insufficient durability of high voltage electrodes. To solve these problems, the water to be treated was dispersed as droplets and sprayed to the high voltage electrodes to make a water drop induced discharge system. The discharge photographs indicated that when dripping down in the discharge gap, water drops can induce the happening of discharge. The discharge channels concentrated near the water drops and the discharge intensity changes with water flow rate. This feature could reduce the requirement for the uniformity of electrodes as the uniform discharge could be obtained by making a uniform water distribution. In addition, both the discharge channels and active species were concentrated on or very close to the water drops to be treated. The transfer distance of active species was shortened, and then both the chemical reaction efficiency and the energy efficiency could be increased. Ibuprofen degradation results showed that the ibuprofen can be removed exceeding 99% after 1 h treatment. The maximum energy yield exceeded 10 g/kWh. Factors including discharge voltage, water flow rate, water conductivity and electrode gap distance influenced the ibuprofen removal. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:708 / 716
页数:9
相关论文
共 28 条
  • [1] Corona Discharge to Water Surface and Its Transition to a Spark
    Bozhko, Igor V.
    Kondratenko, Igor P.
    Serdyuk, Yuriy V.
    [J]. IEEE TRANSACTIONS ON PLASMA SCIENCE, 2011, 39 (05) : 1228 - 1233
  • [2] Bruggeman P., 2008, PLASMA SOURCES SCI T, V17, P969
  • [3] Bruggeman P., 2008, PLASMA SOURCES SCI T, V17, P431
  • [4] Water surface deformation in strong electrical fields and its influence on electrical breakdown in a metal pin-water electrode system
    Bruggeman, Peter
    Graham, Leigh
    Degroote, Joris
    Vierendeels, Jan
    Leys, Christophe
    [J]. JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2007, 40 (16) : 4779 - 4786
  • [5] Modeling of experimental treatment of acetaldehyde-laden air and phenol-containing water using corona discharge technique
    Faungnawakij, K
    Sano, N
    Charinpanitkul, T
    Tanthapanichakoon, W
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006, 40 (05) : 1622 - 1628
  • [6] Corona above water reactor for systematic study of aqueous phenol degradation
    Grabowski, LR
    van Veldhuizen, EM
    Pemen, AJM
    Rutgers, WR
    [J]. PLASMA CHEMISTRY AND PLASMA PROCESSING, 2006, 26 (01) : 3 - 17
  • [7] Hybrid gas-liquid electrical discharge reactors for organic compound degradation
    Grymonpré, DR
    Finney, WC
    Clark, RJ
    Locke, BR
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2004, 43 (09) : 1975 - 1989
  • [8] The Effect of a Water-Droplet Spray and Gas Discharge in Water Treatment by Pulsed Power
    Handa, Taiki
    Minamitani, Yasushi
    [J]. IEEE TRANSACTIONS ON PLASMA SCIENCE, 2009, 37 (01) : 179 - 183
  • [9] Removal of priority pollutants from water by means of dielectric barrier discharge atmospheric plasma
    Hijosa-Valsero, Maria
    Molina, Ricardo
    Schikora, Hendrik
    Mueller, Michael
    Bayona, Josep M.
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2013, 262 : 664 - 673
  • [10] Removal of cyanide from water by means of plasma discharge technology
    Hijosa-Valsero, Maria
    Molina, Ricardo
    Schikora, Hendrik
    Mueller, Michael
    Bayona, Josep M.
    [J]. WATER RESEARCH, 2013, 47 (04) : 1701 - 1707