Modification of polyvinylidene fluoride membrane with different shaped α-Fe2O3 nanocrystals for enhanced photocatalytic oxidation performance

被引:12
作者
Zhang, Enlei [1 ]
Wang, Lijie [1 ]
Zhang, Bengui [1 ]
Xie, Yingpeng [1 ]
Sun, Chuanbi [1 ]
Jiang, Chao [1 ]
Zhang, Ying [1 ]
Wang, Guosheng [1 ]
机构
[1] Shenyang Univ Chem Technol, Coll Chem Engn, Shenyang 110142, Liaoning, Peoples R China
关键词
alpha-Fe2O3; nanorods; Photocatalytic; Membrane process; Polyvinylidene fluoride membrane; VISIBLE-LIGHT; AQUEOUS-SOLUTION; FEOOH NANORODS; PARTICLE-SIZE; FENTON; DEGRADATION; OXIDE; ADSORPTION; CATALYSTS;
D O I
10.1016/j.matchemphys.2018.04.084
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A novel modified polyvinylidene fluoride (PVDF) membranes with adding alpha-Fe2O3 nanocrystals were prepared for the photocatalytic degradation of organic contaminants. The alpha-Fe2O3 nanocrystals entrapped PVDF membranes were characterized by XRD, SEM and TEM. The photocatalytic performance and antifouling property were studied by filtration and degradation of Congo red (CR) under visible light irradiation. The results show that the photocatalytic activity of the alpha-Fe2O3/PVDF membranes were significantly influenced by the morphology of alpha-Fe2O3 nanocrystals. The PVDF membrane with inclusion of alpha-Fe2O3 nanorods showed high degradation efficiency (90%) because of the higher surface Fe3+ density. The water flux and degradation kinetics of the composite membrane were also studied. (C) 2018 Elsevier B.V. All rights reserved.
引用
收藏
页码:41 / 47
页数:7
相关论文
共 30 条
[1]   Recent advances in new generation dye removal technologies: novel search for approaches to reprocess wastewater [J].
Ahmad, Akil ;
Mohd-Setapar, Siti Hamidah ;
Chuong, Chuo Sing ;
Khatoon, Asma ;
Wani, Waseem A. ;
Kumar, Rajeev ;
Rafatullah, Mohd .
RSC ADVANCES, 2015, 5 (39) :30801-30818
[2]   Photoinduced Oxidation of Arsenite to Arsenate in the Presence of Goethite [J].
Bhandari, Narayan ;
Reeder, Richard J. ;
Strongin, Daniel R. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012, 46 (15) :8044-8051
[3]   Dual Enzyme-like Activities of Iron Oxide Nanoparticles and Their Implication for Diminishing Cytotoxicity [J].
Chen, Zhongwen ;
Yin, Jun-Jie ;
Zhou, Yu-Ting ;
Zhang, Yu ;
Song, Lina ;
Song, Mengjie ;
Hu, Sunling ;
Gu, Ning .
ACS NANO, 2012, 6 (05) :4001-4012
[4]   A yolk-shell structured Fe2O3@mesoporous SiO2 nanoreactor for enhanced activity as a Fenton catalyst in total oxidation of dyes [J].
Cui, Zhi-Min ;
Chen, Zhe ;
Cao, Chang-Yan ;
Jiang, Lei ;
Song, Wei-Guo .
CHEMICAL COMMUNICATIONS, 2013, 49 (23) :2332-2334
[5]   Membrane surface modification with TiO2-graphene oxide for enhanced photocatalytic performance [J].
Gao, Yong ;
Hu, Meng ;
Mi, Baoxia .
JOURNAL OF MEMBRANE SCIENCE, 2014, 455 :349-356
[6]   Facile synthesis of magnetic hierarchical MgO-MgFe2O4 composites and their adsorption performance towards Congo red [J].
Han, Xiuying ;
Tian, Peng ;
Pang, Hongchang ;
Song, Qiang ;
Ning, Guiling ;
Yu, Yanhao ;
Fang, Haixia .
RSC ADVANCES, 2014, 4 (53) :28119-28125
[7]   Single-crystalline Bi2Fe4O9 synthesized by low-temperature co-precipitation: performance as photo- and Fenton catalysts [J].
Hu, Zhong-Ting ;
Chen, Bo ;
Lim, Teik-Thye .
RSC ADVANCES, 2014, 4 (53) :27820-27829
[8]   Synthesis of MgFe2O4 nanocrystallites under mild conditions [J].
Huang, YJ ;
Tang, Y ;
Wang, J ;
Chen, QW .
MATERIALS CHEMISTRY AND PHYSICS, 2006, 97 (2-3) :394-397
[9]   Sunlight, iron and radicals to tackle the resistant leftovers of biotreated winery wastewater [J].
Ioannou, Lida ;
Velegraki, Theodora ;
Michael, Costas ;
Mantzavinos, Dionissios ;
Fatta-Kassinos, Despo .
PHOTOCHEMICAL & PHOTOBIOLOGICAL SCIENCES, 2013, 12 (04) :664-670
[10]   A comprehensive review on anti-fouling nanocomposite membranes for pressure driven membrane separation processes [J].
Jhaveri, Jainesh H. ;
Murthy, Z. V. P. .
DESALINATION, 2016, 379 :137-154