Supercontinuum generation in OHQ-N2S organic crystal driven by intense terahertz fields

被引:5
|
作者
Giorgianni, Flavio [1 ]
Puc, Uros [2 ]
Jazbinsek, Mojca [2 ]
Cea, Tommaso [3 ]
Koo, Min-Jeong [4 ]
Han, Jae-Hyun [4 ]
Kwon, O-Pil [4 ]
Vicario, Carlo [1 ]
机构
[1] Paul Scherrer Inst, Lab Nonlinear Opt, Forschungsstr 111, CH-5232 Villigen, Switzerland
[2] Zurich Univ Appl Sci ZHAW, Inst Computat Phys, CH-8401 Winterthur, Switzerland
[3] Imdea Nanosci, Faraday 9, Madrid 28015, Spain
[4] Ajou Univ, Dept Mol Sci & Technol, Suwon 443749, South Korea
基金
瑞士国家科学基金会; 新加坡国家研究基金会;
关键词
THZ PULSES; LIGHT; EMISSION; MATTER;
D O I
10.1364/OL.44.004881
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
A laser supercontinuum is generated by cross-phase modulation (XPM) driven by an intense terahertz (THz) field in organic crystal OHQ-N2S. In this highly nonlinear medium, the THz electric field induces a time-varying optical phase modulation, which causes a spectacular spectral broadening and shifting of a co-propagating near-infrared laser pulse. The effect is enabled by the large electro-optic coefficient, the low absorption, and the good velocity matching between the laser and the THz pulse over the OHQ-N2S crystal thickness. The XPM occurs when the THz field is aligned along the polar axis of the OHQ-N2S. The results display a promising pathway for ultrafast control of the spectral and temporal properties of laser pulses using THz stimuli. (C) 2019 Optical Society of America
引用
收藏
页码:4881 / 4884
页数:4
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