Temperature dependence of intrinsic and extrinsic dielectric contributions in 0.27Pb(In1/2Nb1/2)O3-0.46Pb(Mg1/3Nb2/3)O3-0.27PbTiO3 single crystals

被引：9
|
作者：
Yang, Liya [1 ]
Zheng, Limei [1 ]
Jing, Yujia [1 ]
Li, Shiyang [2 ]
Lu, Xiaoyan [3 ]
Lu, Weiming [1 ]
Zhang, Rui [1 ]
机构：
[1] Harbin Inst Technol, Condensed Matter Sci & Technol Inst, Harbin 150080, Peoples R China
[2] Shanghai Jiao Tong Univ, Dept Instrument Sci & Engn, Shanghai 200240, Peoples R China
[3] Harbin Inst Technol, Sch Civil Engn, Harbin 150001, Peoples R China
来源：
PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS | 2017年 / 254卷 / 07期
基金：
美国国家科学基金会;
关键词：
dielectric properties; ferroelectrics; phase transition; Rayleigh law; single crystals; thermal stability; ZIRCONATE-TITANATE CERAMICS; PIEZOELECTRIC PROPERTIES; THIN-FILMS;
D O I：
10.1002/pssb.201700029
中图分类号：
O469 [凝聚态物理学];
学科分类号：
070205 ;
摘要：
The temperature dependence of extrinsic and intrinsic dielectric contributions was quantitatively evaluated by Rayleigh analysis in [001](C)-oriented rhombohedral 0.27Pb(In1/2Nb1/2)O-3-0.46Pb(Mg1/3Nb2/3)O-3-0.27PbTiO(3) (PIN-PMN-0.27PT) single crystal. It is shown that both contributions increase with temperature and reach maximum values at around the rhombohedral-tetragonal phase-transition temperature TR-T. However, the enhancement of the extrinsic part is more significant than the intrinsic one. The percentage of extrinsic contribution regarding the total dielectric response increases from 1% at room temperature to 34% at around TR-T. In addition, the influence of the polymorphic phase transition on intrinsic and extrinsic contributions is discussed. This work enables us to further understand the thermal stability of electrical properties and the influence of polymorphic phase transition in ferroelectrics.
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页数：5
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