Increasing the Visible Light Absorption of Graphitic Carbon Nitride (Melon) Photocatalysts by Homogeneous Self-Modification with Nitrogen Vacancies

被引：717

作者：

Niu, Ping ^{[1
]}

Yin, Li-Chang ^{[1
]}

Yang, Yong-Qiang ^{[1
,2
]}

Liu, Gang ^{[1
]}

Cheng, Hui-Ming ^{[1
,3
]}

机构：

[1] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China

[2] Univ Sci & Technol China, Sch Chem & Mat Sci, Dept Mat Sci & Technol, Hefei 230026, Peoples R China

[3] King Abdulaziz Univ, Dept Chem, Fac Sci, Jeddah 21589, Saudi Arabia

来源：

ADVANCED MATERIALS | 2014年 / 26卷 / 47期

关键词：

HYDROGEN EVOLUTION; TIO2-BASED PHOTOCATALYSTS; AQUEOUS SUSPENSIONS; TIO2; PHOTOCATALYST; WATER; SEMICONDUCTORS; CATALYSTS; FILMS; PHOTOREACTIVITY; PHOTOSYNTHESIS;

D O I：

10.1002/adma.201404057

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A novel reduced melon photocatalyst with a bandgap of 2.03 eV developed here has a widened visible light absorption range and suppressed radiative recombination of photo-excited charge carriers due to the homogeneous self-modification with nitrogen vacancies. As a consequence, the reduced melon shows a much superior photocatalytic activity compared to the pristine melon in generating center dot OH radicals and degrading the organic pollutant Rhodamine B.

引用

收藏

页码：8046 / 8052

页数：7

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