Screening Supported Amine Sorbents in the Context of Post-combustion Carbon Capture by Vacuum Swing Adsorption

被引：13

作者：

Krishnamurthy, Shreenath ^{[1
]}

Boon, Juriaan ^{[2
]}

Grande, Carlos ^{[1
]}

Lind, Anna ^{[1
]}

Blom, Richard ^{[1
]}

de Boer, Robert ^{[2
]}

Willemsen, Hans ^{[3
]}

de Scheemaker, Gabriel ^{[3
]}

机构：

[1] SINTEF Ind, Forskningsveien 1, N-0373 Oslo, Norway

[2] TNO Sustainable Proc Technol, POB 15, NL-1755 ZG Petten, Netherlands

[3] 3D Cat BV, Kerkelaan 28, NL-1861 EB Bergen, Norway

来源：

CHEMIE INGENIEUR TECHNIK | 2021年 / 93卷 / 06期

关键词：

Energy vs productivity Pareto; Post‐ combustion carbon capture; Process simulation; Supported amine sorbents; Vacuum swing adsorption; METAL-ORGANIC FRAMEWORKS; CO2; CAPTURE; POWER-PLANTS; OPTIMIZATION; ADSORBENTS; SIMULATION; SEPARATION; CYCLE; TEMPERATURE; MEMBRANES;

D O I：

10.1002/cite.202000172

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

The aim of this work was to evaluate the performance of three different supported amine sorbents in a 6-step vacuum swing adsorption (VSA) cycle through process simulation and optimization for a representative post-combustion CO2 capture system. Detailed process optimization revealed that all the adsorbents were able to achieve the desired purity-recovery targets. The best performing adsorbent in terms of productivity was Lewatit with a productivity of 0.48 mol m(-3) ads s(-1). All the adsorbents exhibited similar minimum specific energy value of around 1 MJ kg(-1) on an electric basis.

引用

页码：929 / 940

页数：12

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