Screening Supported Amine Sorbents in the Context of Post-combustion Carbon Capture by Vacuum Swing Adsorption

被引：13
作者：
Krishnamurthy, Shreenath [1 ]
Boon, Juriaan [2 ]
Grande, Carlos [1 ]
Lind, Anna [1 ]
Blom, Richard [1 ]
de Boer, Robert [2 ]
Willemsen, Hans [3 ]
de Scheemaker, Gabriel [3 ]
机构：
[1] SINTEF Ind, Forskningsveien 1, N-0373 Oslo, Norway
[2] TNO Sustainable Proc Technol, POB 15, NL-1755 ZG Petten, Netherlands
[3] 3D Cat BV, Kerkelaan 28, NL-1861 EB Bergen, Norway
来源：
CHEMIE INGENIEUR TECHNIK | 2021年 / 93卷 / 06期
关键词：
Energy vs productivity Pareto; Post‐ combustion carbon capture; Process simulation; Supported amine sorbents; Vacuum swing adsorption; METAL-ORGANIC FRAMEWORKS; CO2; CAPTURE; POWER-PLANTS; OPTIMIZATION; ADSORBENTS; SIMULATION; SEPARATION; CYCLE; TEMPERATURE; MEMBRANES;
D O I：
10.1002/cite.202000172
中图分类号：
TQ [化学工业];
学科分类号：
0817 ;
摘要：
The aim of this work was to evaluate the performance of three different supported amine sorbents in a 6-step vacuum swing adsorption (VSA) cycle through process simulation and optimization for a representative post-combustion CO2 capture system. Detailed process optimization revealed that all the adsorbents were able to achieve the desired purity-recovery targets. The best performing adsorbent in terms of productivity was Lewatit with a productivity of 0.48 mol m(-3) ads s(-1). All the adsorbents exhibited similar minimum specific energy value of around 1 MJ kg(-1) on an electric basis.
引用
收藏
页码：929 / 940
页数：12
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