Characteristics of long-range transported PM2.5 at a coastal city using the single particle aerosol mass spectrometry

被引:5
作者
Cai, Qiuliang [1 ,2 ,3 ]
Tong, Lei [1 ,2 ]
Zhang, Jingjing [1 ,2 ,3 ]
Zheng, Jie [1 ,2 ]
He, Mengmeng [1 ,2 ]
Lin, Jiamei [1 ,2 ,3 ]
Chen, Xiaoqiu [4 ]
Xiao, Hang [1 ,2 ]
机构
[1] Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Fujian, Peoples R China
[2] Chinese Acad Sci, NUEORS, Ningbo 315830, Zhejiang, Peoples R China
[3] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[4] Environm Monitoring Ctr Fujian, Fuzhou 350003, Fujian, Peoples R China
关键词
Particle number; Partide size; PM2.5; PSCF; SPAMS; CHEMICAL-COMPOSITION; SOURCE APPORTIONMENT; PARTICULATE MATTER; SIZE; DISTRIBUTIONS; EXPOSURE; CHINA;
D O I
10.4491/eer.2018.354
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Air pollution has attracted ever-increasing attention because of its substantial influence on air quality and human health. To better understand the characteristics of long-range transported pollution, the single particle chemical composition and size were investigated by the single partide aerosol mass spectrometry in Fuzhou, China from 17th to 22nd January, 2016. The results showed that the haze was mainly caused by the transport of cold air mass under higher wind speed (10 m.s(-1)) from the Yangtze River Delta region to Fuzhou. The number concentration elevated from 1,000 to 4,500 #.h(-1), and the composition of mobile source and secondary aerosol increased from 24.3% to 30.9% and from 16.0% to 22.5%, respectively. Then, the haze was eliminated by the dean air mass from the sea as indicated by a sharp decrease of partide number concentration from 4,500 to 1,000 #.h(-1). The composition of secondary aerosol and mobile sources decreased from 29.3% to 23.5% and from 30.9% to 23.1%, respectively. The particles with the size ranging from 0.5 to 1.5 mu m were mainly in the accumulation mode. The stationary source, mobile source, and secondary aerosol contributed to over 70% of the potential sources. These results will help to understand the physical and chemical characteristics of long- range transported pollutants.
引用
收藏
页码:690 / 698
页数:9
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