Hydrogen-bond dynamics in water explored by heterodyne-detected photon echo

被引：170
|
作者：
Yeremenko, S [1 ]
Pshenichnikov, MS [1 ]
Wiersma, DA [1 ]
机构：
[1] Univ Groningen, Ctr Mat Sci, Ultrafast Laser & Spect Lab, NL-9747 AG Groningen, Netherlands
来源：
CHEMICAL PHYSICS LETTERS | 2003年 / 369卷 / 1-2期
关键词：
D O I：
10.1016/S0009-2614(02)02001-8
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Results of heterodyne-detected photon echo experiments on the OH stretching mode of water are reported and discussed. Two vibrational dynamical processes with time constants of 130 and 900 fs were identified. The former is attributed to bond breaking dynamics of a single hydrogen bond, the latter to rearrangement of the hydrogen-bond network. (C) 2003 Elsevier Science B.V. All rights reserved.
引用
收藏
页码：107 / 113
页数：7
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