Evidence for an H2 promoting effect in the selective catalytic reduction of NOx by propene on Au/Al2O3

被引：16
|
作者：
Chaieb, Tesnim [1 ,2 ]
Delannoy, Laurent [1 ,2 ]
Casale, Sandra [1 ,2 ]
Louis, Catherine [1 ,2 ]
Thomas, Cyril [1 ,2 ]
机构：
[1] Univ Paris 06, Sorbonne Univ, UMR 7197, Lab React Surface, F-75252 Paris, France
[2] CNRS, UMR 7197, Lab React Surface, F-75252 Paris, France
来源：
CHEMICAL COMMUNICATIONS | 2015年 / 51卷 / 04期
关键词：
NITROGEN MONOXIDE; GOLD CATALYSTS; NITRIC-OXIDE; HYDROCARBONS; HYDROGEN; C3H6-SCR; OXYGEN; AL2O3; STEP; AG;
D O I：
10.1039/c4cc07349e
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
This work provides the first experimental evidence of an H-2 effect in C3H6-SCR over an Au/Al2O3 catalyst. This effect could only be observed when the number of Au catalytic sites was decreased. The N-2 turnover rate estimated for the first time for the Au catalytic sites for H-2-C3H6-SCR was found to be similar to that estimated for Ag ones supported on Al2O3.
引用
收藏
页码：796 / 799
页数：4
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