Simultaneous measurement of tritium and radiocarbon by ultra-low-background proportional counting

被引:0
作者
Mace, Emily [1 ]
Aalseth, Craig [1 ]
Alexander, Tom [1 ]
Back, Henning [1 ]
Day, Anthony [1 ]
Hoppe, Eric [1 ]
Keillor, Martin [1 ]
Moran, Jim [1 ]
Overman, Cory [1 ]
Panisko, Mark [1 ]
Seifert, Allen [1 ]
机构
[1] Pacific Northwest Natl Lab, 902 Battelle Blvd,MSIN J4-65, Richland, WA 99352 USA
关键词
Tritium; Radiocarbon; Ultra-low-background; Proportional counting; Dual-isotope measurements; CHEMICAL FORMS; C-14; WATER; METHANE; ENVIRONMENT; FUKUOKA; JAPAN; H-3;
D O I
10.1016/j.apradiso.2016.12.033
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Use of ultra-low-background capabilities at Pacific Northwest National Laboratory provide enhanced sensitivity for measurement of low-activity sources of tritium and radiocarbon using proportional counters. Tritium levels are nearly back to pre-nuclear test backgrounds (similar to 2-8 TU in rainwater), which can complicate their dual measurement with radiocarbon due to overlap in the beta decay spectra. We present results of single-isotope proportional counter measurements used to analyze a dual-isotope methane sample synthesized from similar to 120 mg of H2O and present sensitivity results.
引用
收藏
页码:171 / 174
页数:4
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