Single carbon dioxide molecules on surfaces studied by low-temperature scanning tunneling microscopy

被引：1
作者：
Wang, Yawei [1 ]
Li, Na [1 ]
Wang, Yongfeng [1 ,2 ]
机构：
[1] Peking Univ, Dept Elect, Key Lab Phys & Chem Nanodevices, Beijing 100871, Peoples R China
[2] Peking Univ, Informat Technol Inst Tianjin Binhai, Tianjin 300450, Peoples R China
来源：
RESEARCH ON CHEMICAL INTERMEDIATES | 2017年 / 43卷 / 09期
基金：
中国国家自然科学基金;
关键词：
Scanning tunneling microscopy; Carbon dioxide; Surface chemistry; METAL-ORGANIC FRAMEWORKS; CO2; ADSORPTION; RUTILE TIO2(110); PHOTOCATALYTIC ACTIVITY; CHEMISORPTION; REDUCTION; CATALYSTS; HYDROGEN; NICKEL; H2O;
D O I：
10.1007/s11164-017-3054-9
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
The chemical conversion of carbon dioxide (CO2) has been intensively studied because the molecule is responsible for global warming. Rational design of catalysts plays an important role in converting CO2 into value-added compounds. Understanding the interaction between CO2 and surfaces of catalysts is a prerequisite to preparing high-performance catalysts. This review focuses on the investigations of CO2 molecules on single crystalline surfaces studied by low-temperature scanning tunneling microscopy. Molecular adsorption, diffusion, and conversion on metal surfaces, metal oxide surfaces, and surfaces decorated by metal-organic frameworks are summarized.
引用
收藏
页码：5229 / 5243
页数：15
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共 63 条
  • [1] CO2 Adsorption, Diffusion, and Electron-Induced Chemistry on Rutile TiO2(110): A Low-Temperature Scanning Tunneling Microscopy Study
    Acharya, D. P.
    Camillone, N., III
    Sutter, P.
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (24) : 12095 - 12105
  • [2] CO2 Adsorption As a Flat-Lying, Tridentate Carbonate on CeO2(100)
    Albrecht, Peter M.
    Jiang, De-en
    Mullins, David R.
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2014, 118 (17) : 9042 - 9050
  • [3] OXYGEN INDUCED ADSORPTION AND REACTION OF H-2, H2O, CO AND CO2 ON SINGLE-CRYSTAL AG(110)
    BOWKER, M
    BARTEAU, MA
    MADIX, RJ
    [J]. SURFACE SCIENCE, 1980, 92 (2-3) : 528 - 548
  • [4] CO2 Binding and Induced Structural Collapse of a Surface-Supported Metal-Organic Network
    Cechal, Jan
    Kley, Christopher S.
    Petuya, Remi
    Schramm, Frank
    Ruben, Mario
    Stepanow, Sebastian
    Arnau, Andres
    Kern, Klaus
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2016, 120 (33) : 18622 - 18630
  • [5] Opportunities and prospects in the chemical recycling of carbon dioxide to fuels
    Centi, Gabriele
    Perathoner, Siglinda
    [J]. CATALYSIS TODAY, 2009, 148 (3-4) : 191 - 205
  • [6] Modification of the Mg/DOBDC MOF with Amines to Enhance CO2 Adsorption from Ultradilute Gases
    Choi, Sunho
    Watanabe, Taku
    Bae, Tae-Hyun
    Sholl, David S.
    Jones, Christopher W.
    [J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2012, 3 (09): : 1136 - 1141
  • [7] Transformation of Carbon Dioxide with Homogeneous Transition-Metal Catalysts: A Molecular Solution to a Global Challenge?
    Cokoja, Mirza
    Bruckmeier, Christian
    Rieger, Bernhard
    Herrmann, Wolfgang A.
    Kuehn, Fritz E.
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2011, 50 (37) : 8510 - 8537
  • [8] THE REACTIVE CHEMISORPTION OF CARBON DIOXIDE AT MAGNESIUM AND COPPER SURFACES AT LOW TEMPERATURE
    Copperthwaite, R. G.
    Davies, P. R.
    Morris, M. A.
    Roberts, M. W.
    Ryder, R. A.
    [J]. CATALYSIS LETTERS, 1988, 1 (1-3) : 11 - 19
  • [9] One step towards bridging the materials gap:: surface studies of TiO2 anatase
    Diebold, U
    Ruzycki, N
    Herman, GS
    Selloni, A
    [J]. CATALYSIS TODAY, 2003, 85 (2-4) : 93 - 100
  • [10] Recycling CO2? Computational Considerations of the Activation of CO2 with Homogeneous Transition Metal Catalysts
    Drees, Markus
    Cokoja, Mirza
    Kuehn, Fritz E.
    [J]. CHEMCATCHEM, 2012, 4 (11) : 1703 - 1712
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