Low-Bandgap Mixed Tin-Lead Perovskites and Their Applications in All-Perovskite Tandem Solar Cells

被引：158

作者：

Wang, Changlei ^{[1
,2
,3
,4
,5
]}

Song, Zhaoning ^{[1
,2
]}

Li, Chongwen ^{[1
,2
]}

Zhao, Dewei ^{[1
,2
,6
,7
]}

Yan, Yanfa ^{[1
,2
]}

机构：

[1] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA

[2] Univ Toledo, Wright Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA

[3] Soochow Univ, Sch Optoelect Sci & Engn, Suzhou 215006, Peoples R China

[4] Soochow Univ, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Key Lab Adv Opt Mfg Technol Jiangsu Prov, Suzhou 215006, Peoples R China

[5] Soochow Univ, Key Lab Modern Opt Technol, Educ Minist China, Suzhou 215006, Peoples R China

[6] Nanchang Univ, Ordered Matter Sci Res Ctr, Nanchang 330031, Jiangxi, Peoples R China

[7] Nanchang Univ, Coll Chem, Nanchang 330031, Jiangxi, Peoples R China

来源：

ADVANCED FUNCTIONAL MATERIALS | 2019年 / 29卷 / 47期

关键词：

low bandgaps; mixed tin-lead; perovskite solar cells; tandem solar cells; HOLE TRANSPORTING MATERIAL; HALIDE PEROVSKITES; EFFICIENT PLANAR; HIGHLY EFFICIENT; OPTICAL-PROPERTIES; IODIDE PEROVSKITE; LARGE GRAINS; PERFORMANCE; STABILITY; SN;

D O I：

10.1002/adfm.201808801

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Efficient organic-inorganic metal halide perovskite absorbers have gained tremendous research interest in the past decade due to their super optoelectronic properties and defect tolerance. Lead (Pb) halide perovskites enable highly efficient perovskite solar cells (PSCs) with a record power conversion efficiency (PCE) of over 23%. However, the energy bandgaps of Pb halide perovskites are larger than the optimal bandgap for single junction solar cells, governed by the Shockley-Queisser (SQ) radiative limit. Mixed tin (Sn)-Pb halide perovskites have drawn significant attention, since their bandgap can be tuned to below 1.2 eV, which opens a door for fabricating all-perovskite tandem solar cells that can break the SQ radiative limit. This review summarizes the development of low-bandgap mixed Sn-Pb PSCs and their applications in all-perovskite tandem solar cells. Its aim is to facilitate the development of new approaches to achieve high efficiency low-bandgap single-junction mixed Sn-Pb PSCs and all-perovskite tandem solar cells.

引用

页数：30

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