Impact of P3HT materials properties and layer architecture on OPV device stability

被引：22

作者：

Meitzner, Rico ^{[1
,2
]}

Faber, Tobias ^{[3
]}

Alam, Shahidul ^{[1
,2
]}

Amand, Aman ^{[1
,2
]}

Roesch, Roland ^{[1
,2
]}

Buettner, Mathias ^{[3
]}

Herrmann-Westendorf, Felix ^{[4
]}

Presselt, Martin ^{[1
,4
,20
,21
]}

Ciammaruchi, Laura ^{[5
]}

Visoly-Fisher, Iris ^{[5
,6
]}

Veenstra, Sjoerd ^{[7
]}

de Zerio, Amaia Diaz ^{[8
]}

Xu, Xiaofeng ^{[8
]}

Wang, Ergang ^{[8
]}

Mueller, Christian ^{[8
]}

Troshin, Pavel ^{[9
,10
]}

Hager, Martin D. ^{[1
,2
]}

Koehn, Sandra ^{[1
,2
]}

Dusza, Michal ^{[11
,12
]}

Krassas, Miron ^{[13
]}

Zuefle, Simon ^{[18
,19
]}

Kymakis, E. ^{[13
]}

Katz, Eugene A. ^{[5
,6
]}

Berson, Solenn ^{[14
]}

Granek, Filip ^{[11
]}

Manceau, Matthieu ^{[14
]}

Brunetti, Francesca ^{[15
]}

Polino, Giuseppina ^{[15
]}

Schubert, Ulrich S. ^{[1
,2
]}

Lira-Cantu, Monica ^{[16
,17
]}

Hoppe, Harald ^{[1
,2
]}

机构：

[1] Friedrich Schiller Univ Jena, CEEC Jena, Philosophenweg 7a, D-07743 Jena, Germany

[2] Friedrich Schiller Univ Jena, Lab Organ & Macromol Chem IOMC, Humboldstr 10, D-07743 Jena, Germany

[3] Tech Univ Ilmenau, Inst Phys, Weimarer Str 32, D-98693 Ilmenau, Germany

[4] Friedrich Schiller Univ Jena, Inst Phys Chem, Helmholtzweg 4, D-07743 Jena, Germany

[5] Ben Gurion Univ Negev, J Blaustein Inst Desert Res, Swiss Inst Dryland Environm & Energy Res, Dept Sol Energ & Environm Phys, IL-8499000 Midreshet Ben Gurion, Israel

[6] Ben Gurion Univ Negev, Ilse Katz Inst Nanoscale Sci & Technol, IL-8410501 Beer Sheva, Israel

[7] ECN Solliance, High Tech Campus 21, NL-5656 AE Eindhoven, Netherlands

[8] Chalmers Univ Technol, Dept Chem & Chem Engn, S-41296 Gothenburg, Sweden

[9] Skolkovo Inst Sci & Technol, Nobel St 3, Moscow 121205, Russia

[10] IPCP RAS, Semenov Prospect 1, Chernogolovka 141432, Russia

[11] Wroclaw Res Ctr EIT, Stablowicka 147, PL-54066 Wroclaw, Poland

[12] Polish Acad Sci, Inst Low Temp & Struct Res, Okolna 2, PL-50422 Wroclaw, Poland

[13] Technol Educ Inst TEI Crete, Sch Appl Technol, Ctr Mat Technol & Photon, Elect Engn Dept, Iraklion 71004, Greece

[14] CEA, LITEN DTS, Lab Technol Modules Photovoltaiques, BP 332,50 Ave Lac Leman, F-73377 Le Bourget Du Lac, France

[15] Univ Roma Tor Vergata, Dept Elect Engn, CHOSE, Via Politecn 1, I-00133 Rome, Italy

[16] CSIC, Catalan Inst Nanosci & Nanotechnol ICN2, Bldg ICN2,Campus UAB, E-08193 Barcelona, Spain

[17] Barcelona Inst Sci & Technol, Bldg ICN2,Campus UAB, E-08193 Barcelona, Spain

[18] Zurich Univ Appl Sci ZHAW, Inst Computat Phys, Wildbachstr 21, CH-8400 Winterthur, Switzerland

[19] Fluxim AG, Katharina Sulzer Pl 2, CH-8400 Winterthur, Switzerland

[20] Leibniz Inst Photon Technol IPHT, Albert Einstein Str 9, D-07745 Jena, Germany

[21] Sciclus GmbH & Co KG, Moritz von Rohr Str 1a, D-07745 Jena, Germany

来源：

SOLAR ENERGY MATERIALS AND SOLAR CELLS | 2019年 / 202卷

关键词：

Organic solar cells; P3HT; Stability; ISOS; FULLERENE SOLAR-CELLS; EXTERNAL QUANTUM EFFICIENCY; SUB-BANDGAP ABSORPTION; CONJUGATED POLYMERS; PHOTOCHEMICAL STABILITY; ORGANIC PHOTOVOLTAICS; THERMAL-DEGRADATION; ESR SPECTROSCOPY; BLOCKING LAYER; THIN-FILMS;

D O I：

10.1016/j.solmat.2019.110151

中图分类号：

TE [石油、天然气工业]; TK [能源与动力工程];

学科分类号：

0807 ; 0820 ;

摘要：

We report a cooperative study conducted between different laboratories to investigate organic solar cell degradation with respect to P3HT material properties and different solar cell architectures. Various batches of P3HT were collected from different suppliers reflecting commercial availability as well as properties variability. Among the materials properties explicitly considered were the molar mass, dispersity, regio-regularity, impurities by trace metals and intrinsic doping evaluated from radical concentrations. Each of the participating laboratories contributing test devices applied their own layer stack, i.e. their own device architecture and layout. This variation was appreciated as another parameter for evaluation. Even though a large amount of devices failed due to extrinsic degradation effects, indeed, some materials properties were found to be more important than others for obtaining long lifetimes and high stability of P3HT-based polymer solar cells.

引用

页数：17

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