Nucleation on surfaces and in confinement

被引：33

作者：

Whittaker, Michael L. ^{[1
]}

Dove, Patricia M. ^{[2
]}

Joester, Derk ^{[1
]}

机构：

[1] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA

[2] Virginia Polytech Inst & State Univ, Dept Geosci, Blacksburg, VA 24061 USA

来源：

MRS BULLETIN | 2016年 / 41卷 / 05期

基金：

美国国家科学基金会;

关键词：

CALCITE NUCLEATION; CRYSTAL NUCLEATION; BIOMINERALIZATION; CRYSTALLIZATION; CARBONATE; KINETICS; CLUSTERS; GROWTH; PRECIPITATION; INTERFACES;

D O I：

10.1557/mrs.2016.90

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

A review of recent literature supports the notion that organisms may achieve nanoscale control over the hierarchical assembly of organic-inorganic materials by compartmentalizing reactions into small volumes containing specifically functionalized macromolecules. Such confinement may introduce a degree of determinism to the stochastic process of nucleation by greatly reducing the number of nucleation events, allowing an organism to control nucleation using "soft" organic substrates. In this way, the polymorph, orientation, shape, and size of a crystalline building block can be selected, and its assembly into a larger structure orchestrated by the organic matrix.

引用

页码：388 / 392

页数：5

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