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How important is biological ice nucleation in clouds on a global scale?
被引:218
作者:
Hoose, C.
[1
,2
]
Kristjansson, J. E.
[1
]
Burrows, S. M.
[3
]
机构:
[1] Univ Oslo, Dept Geosci, Oslo, Norway
[2] Karlsruhe Inst Technol, Inst Meteorol & Climate Res, Karlsruhe, Germany
[3] Max Planck Inst Chem, D-55128 Mainz, Germany
来源:
ENVIRONMENTAL RESEARCH LETTERS
|
2010年
/
5卷
/
02期
关键词:
ice nucleation;
biological aerosol;
aerosol-cloud interactions;
CONTACT FREEZING MODES;
ACTIVE BACTERIA;
DIFFERENT ECOSYSTEMS;
ORGANIC-CARBON;
FUNGAL SPORES;
ATMOSPHERE;
PRECIPITATION;
PARTICLES;
AEROSOLS;
CLIMATE;
D O I:
10.1088/1748-9326/5/2/024009
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
The high ice nucleating ability of some biological particles has led to speculations about living and dead organisms being involved in cloud ice and precipitation formation, exerting a possibly significant influence on weather and climate. In the present study, the role of primary biological aerosol particles (PBAPs) as heterogeneous ice nuclei is investigated with a global model. Emission parametrizations for bacteria, fungal spores and pollen based on recent literature are introduced, as well as an immersion freezing parametrization based on classical nucleation theory and laboratory measurements. The simulated contribution of PBAPs to the global average ice nucleation rate is only 10-5%, with an uppermost estimate of 0.6%. At the same time, observed PBAP concentrations in air and biological ice nucleus concentrations in snow are reasonably well captured by the model. This implies that 'bioprecipitation' processes ( snow and rain initiated by PBAPs) are of minor importance on the global scale.
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