共 43 条
Silicon-Carbon composite anodes from industrial battery grade silicon
被引:93
作者:

Andersen, Hanne Flaten
论文数: 0 引用数: 0
h-index: 0
机构:
Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway

论文数: 引用数:
h-index:
机构:

Voje, Jorunn
论文数: 0 引用数: 0
h-index: 0
机构:
Elkem, Oslo, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway

Tronstad, Ragnar
论文数: 0 引用数: 0
h-index: 0
机构:
Elkem, Oslo, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway

Mokkelbost, Tommy
论文数: 0 引用数: 0
h-index: 0
机构:
Elkem, Oslo, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway

ErikVullum, Per
论文数: 0 引用数: 0
h-index: 0
机构:
SINTEF, Trondheim, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway

Ulvestad, Asbjorn
论文数: 0 引用数: 0
h-index: 0
机构:
Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway
Univ Oslo, Dept Phys, Oslo, Norway
Kjeller Univ, Grad Ctr UNIK, Kjeller, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway

Kirkengen, Martin
论文数: 0 引用数: 0
h-index: 0
机构:
Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway
Univ Oslo, Dept Phys, Oslo, Norway
Kjeller Univ, Grad Ctr UNIK, Kjeller, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway

Maehlen, Jan Petter
论文数: 0 引用数: 0
h-index: 0
机构:
Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway
机构:
[1] Inst Energy Technol, POB 40, NO-2027 Kjeller, Norway
[2] Elkem, Oslo, Norway
[3] SINTEF, Trondheim, Norway
[4] Univ Oslo, Dept Phys, Oslo, Norway
[5] Kjeller Univ, Grad Ctr UNIK, Kjeller, Norway
关键词:
SOLID-ELECTROLYTE INTERPHASE;
LITHIUM-ION BATTERIES;
ELECTROCHEMICAL PROPERTIES;
FLUOROETHYLENE CARBONATE;
MILLED SI;
LIFE;
D O I:
10.1038/s41598-019-51324-4
中图分类号:
O [数理科学和化学];
P [天文学、地球科学];
Q [生物科学];
N [自然科学总论];
学科分类号:
07 ;
0710 ;
09 ;
摘要:
In this work, silicon/carbon composites for anode electrodes of Li-ion batteries are prepared from Elkem's Silgrain (R) line. Gentle ball milling is used to reduce particle size of Silgrain, and the resulting Si powder consists of micrometic Si with some impurities. Silicon/carbon composite with CMC/SBR as a dual binder can achieve more than 1200 cycles with a capacity of 1000 mAh g(-1) of Si. This excellent electrochemical performance can be attributed to the use of a buffer as a solvent to control the pH of the electrode slurry, and hence the bonding properties of the binder to the silicon particles. In addition, the use of FEC as an electrolyte additive is greatly contributing to a stabilized cycling by creating a more robust SEI layer. This work clearly demonstrates the potential of industrial battery grade silicon from Elkem.
引用
收藏
页数:9
相关论文
共 43 条
[1]
Understanding capacity fade in silicon based electrodes for lithium-ion batteries using three electrode cells and upper cut-off voltage studies
[J].
Beattie, Shane D.
;
Loveridge, M. J.
;
Lain, Michael J.
;
Ferrari, Stefania
;
Polzin, Bryant J.
;
Bhagat, Rohit
;
Dashwood, Richard
.
JOURNAL OF POWER SOURCES,
2016, 302
:426-430

Beattie, Shane D.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England

Loveridge, M. J.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England

Lain, Michael J.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England

论文数: 引用数:
h-index:
机构:

Polzin, Bryant J.
论文数: 0 引用数: 0
h-index: 0
机构:
Argonne Natl Lab, CAMP Cell Anal Modelling & Prototyping Facil, Argonne, IL 60439 USA
Argonne Natl Lab, Support Grp, Argonne, IL 60439 USA Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England

Bhagat, Rohit
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England

论文数: 引用数:
h-index:
机构:
[2]
A novel slurry concept for the fabrication of lithium-ion battery electrodes with beneficial properties
[J].
Bitsch, Boris
;
Dittmann, Jens
;
Schmitt, Marcel
;
Schaffer, Philip
;
Schabel, Wilhelm
;
Willenbacher, Norbert
.
JOURNAL OF POWER SOURCES,
2014, 265
:81-90

Bitsch, Boris
论文数: 0 引用数: 0
h-index: 0
机构:
Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany

Dittmann, Jens
论文数: 0 引用数: 0
h-index: 0
机构:
Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany

Schmitt, Marcel
论文数: 0 引用数: 0
h-index: 0
机构:
Karlsruhe Inst Technol, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany

Schaffer, Philip
论文数: 0 引用数: 0
h-index: 0
机构:
Karlsruhe Inst Technol, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany

Schabel, Wilhelm
论文数: 0 引用数: 0
h-index: 0
机构:
Karlsruhe Inst Technol, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany

Willenbacher, Norbert
论文数: 0 引用数: 0
h-index: 0
机构:
Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Inst Mech Proc Engn & Mech, D-76131 Karlsruhe, Germany
[3]
High capacity lithium ion battery anodes of silicon and germanium
[J].
Bogart, Timothy D.
;
Chockla, Aaron M.
;
Korgel, Brian A.
.
CURRENT OPINION IN CHEMICAL ENGINEERING,
2013, 2 (03)
:286-293

Bogart, Timothy D.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Texas Austin, Dept Chem Engn, Ctr Nano & Mol Sci & Technol, Texas Mat Inst, Austin, TX 78712 USA Univ Texas Austin, Dept Chem Engn, Ctr Nano & Mol Sci & Technol, Texas Mat Inst, Austin, TX 78712 USA

Chockla, Aaron M.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Texas Austin, Dept Chem Engn, Ctr Nano & Mol Sci & Technol, Texas Mat Inst, Austin, TX 78712 USA Univ Texas Austin, Dept Chem Engn, Ctr Nano & Mol Sci & Technol, Texas Mat Inst, Austin, TX 78712 USA

Korgel, Brian A.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Texas Austin, Dept Chem Engn, Ctr Nano & Mol Sci & Technol, Texas Mat Inst, Austin, TX 78712 USA Univ Texas Austin, Dept Chem Engn, Ctr Nano & Mol Sci & Technol, Texas Mat Inst, Austin, TX 78712 USA
[4]
Silicon nanowire anode: Improved battery life with capacity-limited cycling
[J].
Chakrapani, Vidhya
;
Rusli, Florencia
;
Filler, Michael A.
;
Kohl, Paul A.
.
JOURNAL OF POWER SOURCES,
2012, 205
:433-438

Chakrapani, Vidhya
论文数: 0 引用数: 0
h-index: 0
机构:
Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA

Rusli, Florencia
论文数: 0 引用数: 0
h-index: 0
机构:
Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA

Filler, Michael A.
论文数: 0 引用数: 0
h-index: 0
机构:
Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA

Kohl, Paul A.
论文数: 0 引用数: 0
h-index: 0
机构:
Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA
[5]
Surface chemistry and morphology of the solid electrolyte interphase on silicon nanowire lithium-ion battery anodes
[J].
Chan, Candace K.
;
Ruffo, Riccardo
;
Hong, Seung Sae
;
Cui, Yi
.
JOURNAL OF POWER SOURCES,
2009, 189 (02)
:1132-1140

Chan, Candace K.
论文数: 0 引用数: 0
h-index: 0
机构:
Stanford Univ, Dept Chem, Stanford, CA 94305 USA Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA

论文数: 引用数:
h-index:
机构:

Hong, Seung Sae
论文数: 0 引用数: 0
h-index: 0
机构:
Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA

Cui, Yi
论文数: 0 引用数: 0
h-index: 0
机构:
Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
[6]
Effect of fluoroethylene carbonate additive on interfacial properties of silicon thin-film electrode
[J].
Choi, Nam-Soon
;
Yew, Kyoung Han
;
Lee, Kyu Youl
;
Sung, Minseok
;
Kim, Ho
;
Kim, Sung-Soo
.
JOURNAL OF POWER SOURCES,
2006, 161 (02)
:1254-1259

Choi, Nam-Soon
论文数: 0 引用数: 0
h-index: 0
机构:
Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea

Yew, Kyoung Han
论文数: 0 引用数: 0
h-index: 0
机构:
Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea

Lee, Kyu Youl
论文数: 0 引用数: 0
h-index: 0
机构:
Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea

Sung, Minseok
论文数: 0 引用数: 0
h-index: 0
机构:
Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea

Kim, Ho
论文数: 0 引用数: 0
h-index: 0
机构:
Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea

Kim, Sung-Soo
论文数: 0 引用数: 0
h-index: 0
机构:
Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea Samsung SDI Co Ltd, Corp R&D Ctr, Yongin 446577, South Korea
[7]
A low-cost and high performance ball-milled Si-based negative electrode for high-energy Li-ion batteries
[J].
Gauthier, Magali
;
Mazouzi, Driss
;
Reyter, David
;
Lestriez, Bernard
;
Moreau, Philippe
;
Guyomard, Dominique
;
Roue, Lionel
.
ENERGY & ENVIRONMENTAL SCIENCE,
2013, 6 (07)
:2145-2155

Gauthier, Magali
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France
INRS Energie Mat & Telecommun, Varennes, PQ J3X 1S2, Canada Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France

论文数: 引用数:
h-index:
机构:

Reyter, David
论文数: 0 引用数: 0
h-index: 0
机构:
INRS Energie Mat & Telecommun, Varennes, PQ J3X 1S2, Canada Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France

论文数: 引用数:
h-index:
机构:

Moreau, Philippe
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France

Guyomard, Dominique
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France

Roue, Lionel
论文数: 0 引用数: 0
h-index: 0
机构:
INRS Energie Mat & Telecommun, Varennes, PQ J3X 1S2, Canada Univ Nantes, Inst Mat Jean Rouxel IMN, CNRS, F-44322 Nantes 3, France
[8]
Three dimensional studies of particle failure in silicon based composite electrodes for lithium ion batteries
[J].
Gonzalez, Joseph
;
Sun, Ke
;
Huang, Meng
;
Lambros, John
;
Dillon, Shen
;
Chasiotis, Ioannis
.
JOURNAL OF POWER SOURCES,
2014, 269
:334-343

Gonzalez, Joseph
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Illinois, Dept Aerosp Engn, Champaign, IL USA Univ Illinois, Dept Aerosp Engn, Champaign, IL USA

Sun, Ke
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Illinois, Dept Mat Sci & Engn, Champaign, IL USA Univ Illinois, Dept Aerosp Engn, Champaign, IL USA

Huang, Meng
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Illinois, Dept Mat Sci & Engn, Champaign, IL USA Univ Illinois, Dept Aerosp Engn, Champaign, IL USA

Lambros, John
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Illinois, Dept Aerosp Engn, Champaign, IL USA Univ Illinois, Dept Aerosp Engn, Champaign, IL USA

Dillon, Shen
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Illinois, Dept Mat Sci & Engn, Champaign, IL USA Univ Illinois, Dept Aerosp Engn, Champaign, IL USA

Chasiotis, Ioannis
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Illinois, Dept Aerosp Engn, Champaign, IL USA Univ Illinois, Dept Aerosp Engn, Champaign, IL USA
[9]
Lithium alloy negative electrodes
[J].
Huggins, RA
.
JOURNAL OF POWER SOURCES,
1999, 81
:13-19

Huggins, RA
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Kiel, D-24143 Kiel, Germany Univ Kiel, D-24143 Kiel, Germany
[10]
SEI-component formation on sub 5 nm sized silicon nanoparticles in Li-ion batteries: the role of electrode preparation, FEC addition and binders
[J].
Jaumann, Tony
;
Balach, Juan
;
Klose, Markus
;
Oswald, Steffen
;
Langklotz, Ulrike
;
Michaelis, Alexander
;
Eckerta, Juergen
;
Giebeler, Lars
.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS,
2015, 17 (38)
:24956-24967

Jaumann, Tony
论文数: 0 引用数: 0
h-index: 0
机构:
Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany

论文数: 引用数:
h-index:
机构:

Klose, Markus
论文数: 0 引用数: 0
h-index: 0
机构:
Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany

Oswald, Steffen
论文数: 0 引用数: 0
h-index: 0
机构:
Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany

Langklotz, Ulrike
论文数: 0 引用数: 0
h-index: 0
机构:
Tech Univ Dresden, Inst Werkstoffwissensch, D-01069 Dresden, Germany Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany

论文数: 引用数:
h-index:
机构:

Eckerta, Juergen
论文数: 0 引用数: 0
h-index: 0
机构:
Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany
Tech Univ Dresden, Inst Werkstoffwissensch, D-01069 Dresden, Germany Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany

Giebeler, Lars
论文数: 0 引用数: 0
h-index: 0
机构:
Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany
Tech Univ Dresden, Inst Werkstoffwissensch, D-01069 Dresden, Germany Leibniz Inst Solid State & Mat Res IFW Dresden eV, Inst Complex Mat, POB 27 01 16, D-01171 Dresden, Germany